Evidence map›Paper›PMID 35513501›Full record

ArticleNature materials2022

Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology.

Lei Zhu, Ming Zhang, Jinqiu Xu, Chao Li, Jun Yan, Guanqing Zhou, Wenkai Zhong, Tianyu Hao, Jiali Song, Xiaonan Xue and 10 more

Abstract read
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In one paragraph

Article in Nature materials, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 232 papers.

0numbers the graph read from it
0cells of the map it votes in
232citing papers in PubMed
210.8field-weighted citation impact, top 1% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

232 citing papers in PubMed, 2,346 citations in OpenAlex.

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172 more citing papers are in PubMed but not listed here.

4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

20 authors at 6 institutions in 2 countries.

Lei Zhu *Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.ORCID http://orcid.org/0000-0003-3971-0299
Ming Zhang *Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.ORCID http://orcid.org/0000-0002-8101-5487
Jinqiu Xu *Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Chao LiSchool of Chemistry, Beihang University, Beijing, China.
Jun YanDepartment of Physics, Imperial College London, London, UK. j.yan17@imperial.ac.uk.ORCID http://orcid.org/0000-0001-9966-4357
Guanqing ZhouFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Wenkai ZhongFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Tianyu HaoFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Jiali SongSchool of Chemistry, Beihang University, Beijing, China.
Xiaonan XueFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Zichun ZhouFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Rui ZengFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Haiming ZhuDepartment of Chemistry, Zhejiang University, Hangzhou, China.ORCID http://orcid.org/0000-0001-7747-9054
Chun-Chao ChenSchool of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai, China.
Roderick C I MacKenzieDepartment of Engineering, Durham University, Durham, UK.
Yecheng ZouState Key Laboratory of Fluorinated Functional Membrane Materials and Dongyue Future Hydrogen Energy Materials Company, Zibo, China.
Jenny NelsonDepartment of Physics, Imperial College London, London, UK.ORCID http://orcid.org/0000-0003-1048-1330
Yongming ZhangFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China.
Yanming SunSchool of Chemistry, Beihang University, Beijing, China. sunym@buaa.edu.cn.ORCID http://orcid.org/0000-0001-7839-3199
Feng LiuFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China. fengliu82@sjtu.edu.cn.ORCID http://orcid.org/0000-0002-5572-8512
Shanghai Jiao Tong University · CNBeihang University · CNDurham University · GBImperial College London · GBNIHR Imperial Biomedical Research Centre · GBZhejiang University · CN

Funding

National Natural Science Foundation of China (National Science Foundation of China) 21905102National Natural Science Foundation of China (National Science Foundation of China) 22109094National Natural Science Foundation of China (National Science Foundation of China) 51825301, 21734001National Natural Science Foundation of China (National Science Foundation of China) 51973110, 21734009Natural Science Foundation of Shandong Province (Shandong Provincial Natural Science Foundation) ZR2019LFG005
6 · The paper itself

Abstract

In organic photovoltaics, morphological control of donor and acceptor domains on the nanoscale is the key for enabling efficient exciton diffusion and dissociation, carrier transport and suppression of recombination losses. To realize this, here, we demonstrated a double-fibril network based on a ternary donor-acceptor morphology with multi-length scales constructed by combining ancillary conjugated polymer crystallizers and a non-fullerene acceptor filament assembly. Using this approach, we achieved an average power conversion efficiency of 19.3% (certified 19.2%). The success lies in the good match between the photoelectric parameters and the morphological characteristic lengths, which utilizes the excitons and free charges efficiently. This strategy leads to an enhanced exciton diffusion length and a reduced recombination rate, hence minimizing photon-to-electron losses in the ternary devices as compared to their binary counterparts. The double-fibril network morphology strategy minimizes losses and maximizes the power output, offering the possibility of 20% power conversion efficiencies in single-junction organic photovoltaics.

Identifiers

PMID35513501
OpenAlexW4229013424

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.