ArticleACS catalysis2022
Radical Aza-Heck Cyclization of Imidates via Energy Transfer, Electron Transfer, and Cobalt Catalysis.
Article in ACS catalysis, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed, 26 citations in OpenAlex.
- Cobaloxime-catalysed regiodivergent hydrogen atom transfer for alkenyl and allylic carbamoylation with branched alkenes.Nature communications · 2026Article
- Enantioselective rapid assembly of bis-heterocycles by sequential palladium-catalyzed aza-Heck cyclization coupling reaction.Science advances · 2026Article
- Preparation of (Z)-Organic syntheses; an annual publication of satisfactory methods for the preparation of organic chemicals · 2025Article
- Asymmetric imino-acylation of alkenes enabled by HAT-photo/nickel cocatalysis.Chemical science · 2023Article
- Pd(II)-Catalyzed Aminoacetoxylation of Alkenes Via Tether Formation.Organic letters · 2022Article
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
Abstract
A radical aza-Heck cyclization has been developed to afford functionally rich products with four contiguous C-heteroatom bonds. This multi-catalytic strategy provides rapid syntheses of dense, medicinally relevant motifs by enabling the conversion of alcohol-derived imidates to heteroatom-rich fragments containing vinyl oxazolines/oxazoles, allyl amines, β-amino alcohols/halides, and combinations thereof. Mechanistic insights of this process show how three distinct photocatalytic cycles cooperate to enable: (1) imidate radical generation by energy transfer, (2) dehydrogenation by Co catalysis, and (3) catalyst turnover by electron transfer.
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Registered trials
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