ArticleNature communications2022
Defects engineering simultaneously enhances activity and recyclability of MOFs in selective hydrogenation of biomass.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Defect-Rich 2D Layered Double Hydroxides Enhance Sonodynamic Antibacterial Therapy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Synthesis of iron-based metal-organic framework@bacterial cellulose aerogels by anRSC advances · 2025Article
- Application of heterogeneous catalysts in the preparation of bio-based platform compound 5-hydroxymethylfurfural.Bioresources and bioprocessing · 2025Review
- Tuning the electronic states of Pd(II) defect-engineered metal-organic framework catalysts for efficient conversion of isocyanides.Communications chemistry · 2025Article
- Synthetic and analytical considerations for the preparation of amorphous metal-organic frameworks.Chemical science · 2024Review
- Probing Structural Defects in MOFs Using Water Stability.The journal of physical chemistry. C, Nanomaterials and interfaces · 2024Article
- Manipulation of interfacial charge dynamics for metal-organic frameworks toward advanced photocatalytic applications.Nanoscale advances · 2024Review
- Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis.Chemical reviews · 2023Review
- Solvent-derived defects suppress adsorption in MOF-74.Nature communications · 2023Article
- Exploring the Potential of a Highly Scalable Metal-Organic Framework CALF-20 for Selective Gas Adsorption at Low Pressure.Polymers · 2023Article
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8 authors.
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Abstract
The development of synthetic methodologies towards enhanced performance in biomass conversion is desirable due to the growing energy demand. Here we design two types of Ru impregnated MIL-100-Cr defect engineered metal-organic frameworks (Ru@DEMOFs) by incorporating defective ligands (DLs), aiming at highly efficient catalysts for biomass hydrogenation. Our results show that Ru@DEMOFs simultaneously exhibit boosted recyclability, selectivity and activity with the turnover frequency being about 10 times higher than the reported values of polymer supported Ru towards D-glucose hydrogenation. This work provides in-depth insights into (i) the evolution of various defects in the cationic framework upon DLs incorporation and Ru impregnation, (ii) the special effect of each type of defects on the electron density of Ru nanoparticles and activation of reactants, and (iii) the respective role of defects, confined Ru particles and metal single active sites in the catalytic performance of Ru@DEMOFs for D-glucose selective hydrogenation as well as their synergistic catalytic mechanism.
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