ArticleThe journal of physical chemistry. A2022
Spinning-Driven Dynamic Nuclear Polarization with Optical Pumping.
Article in The journal of physical chemistry. A, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- A Qualitative Approach for Predicting Enhanced Intersystem Crossing in Chromophore-Radical Systems.The journal of physical chemistry letters · 2026Article
- Coherent Control over Nuclear Hyperpolarization Using an Optically Initializable Chromophore-Radical System.Journal of the American Chemical Society · 2025Article
- Light-InducedJournal of the American Chemical Society · 2024Article
- Large cross-effect dynamic nuclear polarisation enhancements with kilowatt inverting chirped pulses at 94 GHz.Communications chemistry · 2023Article
- Optically Enhanced Solid-StateJournal of the American Chemical Society · 2023Article
Corrections and comments
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Authors and funding
4 authors.
Funding
Abstract
We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the cross-effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate optical hyperpolarization in the solid state at low temperatures and low field and then investigate its field dependence to obtain the optimal condition for high-field electron spin hyperpolarization. The results are then incorporated into advanced magic-angle spinning dynamic nuclear polarization (MAS-DNP) numerical simulations that show that optically pumped MAS-DNP could yield breakthrough enhancements at very high magnetic fields. Based on these investigations, enhancements greater than the ratio of electron to nucleus magnetic moments (>658 for
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Registered trials
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