ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2022
Unveiling the Synergistic Effect of Ferroelectric Polarization and Domain Configuration for Reversible Zinc Metal Anodes.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Sustainable and Multifunctional Natural Macromolecular Polymers for Aqueous Zn Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Stable Zinc Metal Battery Development: Using Fibrous Zirconia for Rapid Surface Conduction of Zinc Ions With Modified Water Solvation Structure.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Rescuing zinc anode-electrolyte interface: mechanisms, theoretical simulations andChemical science · 2024Review
- Active Dendrite Suppression by Ferroelectric Membrane Separators in Rechargeable Batteries.Nano letters · 2024Article
- Interface Reversible Electric Field Regulated by Amphoteric Charged Protein-Based Coating Toward High-Rate and Robust Zn Anode.Nano-micro letters · 2022Article
- Unveiling the Synergistic Effect of Ferroelectric Polarization and Domain Configuration for Reversible Zinc Metal Anodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2022Article
Corrections and comments
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Authors and funding
6 authors.
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Abstract
The tendency of zinc (Zn) anodes to form uncontrolled Zn electrodeposits and the occurrence of side-reactions at Zn-electrolyte interfaces are a fundamental barrier hampering broad applications of aqueous rechargeable Zn-based batteries. Herein, a ferroelectric domain-mediated strategy is proposed to manipulate the Zn plating behavior and achieve controllable Zn growth orientation by coating Zn foil with a ferroelectric tetragonal KTN (t-KTN) layer. The ferroelectric domain of t-KTN single crystals exhibits periodic distribution of upward and downward polarizations, corresponding to alternating positively and negatively charged surfaces. The charged ferroelectric surfaces can manipulate the transfer kinetics of Zn ions and the concentration distribution of anions via the interplay between ferroelectric dipoles and adsorbed ions. With the synergistic effect of the ferroelectric polarization and domain configurations, the well-aligned interlamellar arrays composed of electrodeposited Zn are formed in the initial deposition process, which enable selective deposition within interlamellar arrays and eliminate the dendrite growth during the following plating process. As a result, the t-KTN layer-modified Zn anode enables reversible Zn plating/stripping with low voltage hysteresis for over 1200 h at 1 mA cm
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