ArticleJournal of the American Chemical Society2022
Electrosynthesis of Biocompatible Free-Standing PEDOT Thin Films at a Polarized Liquid|Liquid Interface.
Article in Journal of the American Chemical Society, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed.
- Multifunctional Conductive Polymer Nanocomposite for Intelligent Pesticide Sensing: Trends, Challenges, and Future Prospects.Molecules (Basel, Switzerland) · 2026Review
- Electropolymerization of Au nanoparticle incorporated poly(dopamine) thin-films at a micro liquid|liquid interface.Nanoscale advances · 2026Article
- Electropolymerization of Organic Mixed Ionic-Electronic Conductors: Fundamentals and Applications in Bioelectronics.Chemical reviews · 2026Review
- Antigravity confined interfacial self-assembly approach for the synthesis and characterization of nanofilms.Nature communications · 2026Article
- Multifunctional Composite Coating-Enhanced Flexible Microelectrodes for Chronic, High-Fidelity Neural Signal Recording.Analytical chemistry · 2025Article
- Engineering Poly(lactic Acid)-Based Scaffolds for Abundant, Sustained, and Prolonged Lactate Release.ACS polymers Au · 2025Article
- Stretchable all-gel organic electrochemical transistors.Nature communications · 2025Article
- Decellularized Biohybrid Nerve Promotes Motor Axon Projections.Advanced healthcare materials · 2024Article
- Comparison of Au Nanoparticle/Poly(9-vinylcarbazole) Thin-Film Electrogeneration at 3 Distinct Liquid/Liquid Interfaces: Water/1,2-Dichloroethane, /α,α,α-Trifluorotoluene, Or/Ionic Liquid.Langmuir : the ACS journal of surfaces and colloids · 2024Article
- Mechanistic Insights into the Potentiodynamic Electrosynthesis of PEDOT Thin Films at a Polarizable Liquid|Liquid Interface.Journal of the American Chemical Society · 2024Article
- In Situ Engineering of Conducting Polymer Nanocomposites at Liquid/Liquid Interfaces: A Perspective on Fundamentals to Technological Significance.ACS materials Au · 2024Review
- Cobalt Oxide 2D Nanosheets Formed at a Polarized Liquid|Liquid Interface toward High-Performance Li-Ion and Na-Ion Battery Anodes.ACS applied materials & interfaces · 2023Article
- Direct imaging of micrometer-thick interfaces in salt-salt aqueous biphasic systems.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Preparation and Characterization of Functionalized Surgical Meshes for Early Detection of Bacterial Infections.ACS biomaterials science & engineering · 2023Article
- Potential-Modulated Ion Distributions in the Back-to-Back Electrical Double Layers at a Polarised Liquid|Liquid Interface Regulate the Kinetics of Interfacial Electron Transfer.ChemElectroChem · 2023Article
- Simultaneous electro-generation/polymerization of Cu nanocluster embedded conductive poly(2,2':5',2''-terthiophene) films at micro and macro liquid/liquid interfaces.Scientific reports · 2023Article
- Why PEDOT:PSS Should Not Be Used for Raman Sensing of Redox States (and How It Could Be).ACS applied materials & interfaces · 2022Article
- Electrodeless Synthesis of Low Dispersity Au Nanoparticles and Nanoclusters at an Immiscible Micro Water/Ionic Liquid Interface.Nanomaterials (Basel, Switzerland) · 2022Article
Corrections and comments
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Authors and funding
10 authors.
Funding
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Abstract
Conducting polymers (CPs) find applications in energy conversion and storage, sensors, and biomedical technologies once processed into thin films. Hydrophobic CPs, like poly(3,4-ethylenedioxythiophene) (PEDOT), typically require surfactant additives, such as poly(styrenesulfonate) (PSS), to aid their aqueous processability as thin films. However, excess PSS diminishes CP electrochemical performance, biocompatibility, and device stability. Here, we report the electrosynthesis of PEDOT thin films at a polarized liquid|liquid interface, a method nonreliant on conductive solid substrates that produces free-standing, additive-free, biocompatible, easily transferrable, and scalable 2D PEDOT thin films of any shape or size in a single step at ambient conditions. Electrochemical control of thin film nucleation and growth at the polarized liquid|liquid interface allows control over the morphology, transitioning from 2D (flat on both sides with a thickness of <50 nm) to "Janus" 3D (with flat and rough sides, each showing distinct physical properties, and a thickness of >850 nm) films. The PEDOT thin films were
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