ArticleACS central science2022
Homogeneously Mixing Different Metal-Organic Framework Structures in Single Nanocrystals through Forming Solid Solutions.
Article in ACS central science, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Eliminating the negative pore synergy in hierarchical porous metal-organic frameworks for isomer separation.Nature communications · 2026Article
- Sequence controlled MOF-on-MOF microcrystals for multidomain liquid chromatography stationary phases.Chemical science · 2026Article
- Highly Selective Adsorption of Para-Xylene, Ethylbenzene, and Explicit Exclusion of Ortho-Xylene from Xylene Isomers Using a Pillar-Layered MOF with Tuned Pore Channels.Angewandte Chemie (International ed. in English) · 2025Article
- Atomically resolved imaging of radiation-sensitive metal-organic frameworks via electron ptychography.Nature communications · 2025Article
- Enhancing Drug Delivery Efficacy Through Bilayer Coating of Zirconium-Based Metal-Organic Frameworks: Sustained Release and Improved Chemical Stability and Cellular Uptake for Cancer Therapy.Chemistry of materials : a publication of the American Chemical Society · 2024Article
- [Rational design of high performance metal organic framework stationary phase for gas chromatography].Se pu = Chinese journal of chromatography · 2023Article
- Anisotropic flexibility and rigidification in a TPE-based Zr-MOFs with scu topology.Nature communications · 2023Article
- Pore Engineering for High Performance Porous Materials.ACS central science · 2023Article
- Two-in-One MOF Structure with Tunable Porosity for Enhanced Separation.ACS central science · 2022Article
Corrections and comments
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Authors and funding
11 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Pore engineering plays a significant role in the applications of porous materials, especially in the area of separation and catalysis. Here, we demonstrated a metal-organic framework (MOF) solid solution (MOSS) strategy to homogeneously and controllably mix NU-1000 and NU-901 structures inside single MOF nanocrystals. The key for the homogeneous mixing and forming of MOSS was the bidentate modulator, which was designed to have a slightly longer distance between two carboxylate groups than the original tetratopic ligand. All of the MOSS nanocrystals showed a uniform pore size distribution with a well-tuned ratio of mesopores to micropores. Because of the appropriate pore ratio, MOSS nanocrystals can balance the thermodynamic interactions and kinetic diffusion of the substrates, thus showing exceedingly higher separation abilities and a unique elution sequence. Our work proposes a rational strategy to design mixed-porous MOFs with controlled pore ratios and provides a new direction to design homogeneously mixed MOFs with a high separation ability and unique separation selectivity.
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Registered trials
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