ArticleScientific reports2022
New paradigm for configurational entropy in glass-forming systems.
Article in Scientific reports, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Critical and Glassy Dualism in Glass-Forming E7 Nematogenic Mixture and Fullerene CNanomaterials (Basel, Switzerland) · 2026Article
- Direct assessment of ionic liquid fragility from transport property variation at moderate temperatures.RSC advances · 2026Article
- Role of Structural Changes at Vitrification and Glass-Liquid Transition.Materials (Basel, Switzerland) · 2025Review
- The Impact of Nanoparticles on Previtreous Behavior: Glass-Forming Nematogenic E7 Mixture-Based Nanocolloids.Nanomaterials (Basel, Switzerland) · 2025Article
- Helical peptide structure improves conductivity and stability of solid electrolytes.Nature materials · 2024Article
- Are Critical Fluctuations Responsible for Glass Formation?Materials (Basel, Switzerland) · 2024Article
- Critical Insight into Pretransitional Behavior and Dielectric Tunability of Relaxor Ceramics.Materials (Basel, Switzerland) · 2023Article
- Phase Equilibria and Critical Behavior in Nematogenic MBBA-Isooctane Monotectic-Type Mixtures.International journal of molecular sciences · 2023Article
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Authors and funding
3 authors.
Funding
Abstract
We show that on cooling towards glass transition configurational entropy exhibits more significant changes than predicted by classic relation. A universal formula according to Kauzmann temperature [Formula: see text] is given: [Formula: see text], where [Formula: see text]. The exponent [Formula: see text] is hypothetically linked to dominated local symmetry. Such a behaviour is coupled to previtreous evolution of heat capacity [Formula: see text] associated with finite temperature singularity. These lead to generalised VFT relation, for which the basic equation is retrieved. For many glass-formers, basic VFT equation may have only an effective meaning. A universal-like reliability of the Stickel operator analysis for detecting dynamic crossover phenomenon is also questioned. Notably, distortions-sensitive and derivative-based analysis focused on previtreous changes of configurational entropy and heat capacity for glycerol, ethanol and liquid crystal is applied.
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Registered trials
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