ArticleNature chemistry2022
Tunable angle-dependent electrochemistry at twisted bilayer graphene with moiré flat bands.
Article in Nature chemistry, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 32 papers.
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Who cites it
32 citing papers in PubMed.
- Engineering Dirac Cones in Graphene for Efficient Iodide Catalysis: Insights by Nanoscale Electrochemistry.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Dynamic twisting and imaging of moiré crystals.Science advances · 2026Article
- Twist-Angle-Dependent Electrocatalytic Activation of Basal Plane MoSMaterials (Basel, Switzerland) · 2026Article
- Chirality Engineering and Properties in Two-Dimensional Layered Materials.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Article
- Polarization-Tunable Photoelectrochemistry at Individual Anisotropic ReSThe journal of physical chemistry letters · 2026Article
- Stacking Order-Mediated Spin-State Modulation in Iron Phthalocyanine Covalent Organic Frameworks Enables Efficient Oxygen Reduction Reaction.ACS applied materials & interfaces · 2026Article
- Moiré-Induced Enhanced Hydrogen Adsorption on Graphene.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Quantum geometry in hexagonal circuit QED lattice with triple leg stripline resonators.Scientific reports · 2025Article
- Roadmap for Photonics with 2D Materials.ACS photonics · 2025Review
- Strain Engineering of Twisted Bilayer Graphene: The Rise of Strain-Twistronics.Small (Weinheim an der Bergstrasse, Germany) · 2025Review
- Sliding Ferroelectric Catalyst for Carbon Nanoparticle Generation.ACS applied nano materials · 2025Article
- Perspectives on electron transfer kinetics across graphene-family nanomaterials and interplay of electronic structure with defects and quantum capacitance.Scientific reports · 2025Article
- Thermal biasing for lattice symmetry breaking and topological edge state imaging.Nature communications · 2025Article
- Electrical monitoring of single-event protonation dynamics at the solid-liquid interface and its regulation by external mechanical forces.Nature communications · 2024Article
- Moiré superlattices in twisted two-dimensional halide perovskites.Nature materials · 2024Article
- Axially Growing Carbon Quantum Ribbon with 2D Stacking Control for High-Stability Solar Cell.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Modeling Scanning Electrochemical Cell Microscopy (SECCM) in Twisted Bilayer Graphene.The journal of physical chemistry letters · 2024Article
- Twisto-Electrochemical Activity Volcanoes in Trilayer Graphene.Journal of the American Chemical Society · 2024Article
- Controlled Formation of Nanoribbons and Their Heterostructures via Assembly of Mass-Selected Inorganic Ions.Advanced materials (Deerfield Beach, Fla.) · 2024Article
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12 authors.
Funding
Abstract
Tailoring electron transfer dynamics across solid-liquid interfaces is fundamental to the interconversion of electrical and chemical energy. Stacking atomically thin layers with a small azimuthal misorientation to produce moiré superlattices enables the controlled engineering of electronic band structures and the formation of extremely flat electronic bands. Here, we report a strong twist-angle dependence of heterogeneous charge transfer kinetics at twisted bilayer graphene electrodes with the greatest enhancement observed near the 'magic angle' (~1.1°). This effect is driven by the angle-dependent tuning of moiré-derived flat bands that modulate electron transfer processes with the solution-phase redox couple. Combined experimental and computational analysis reveals that the variation in electrochemical activity with moiré angle is controlled by a structural relaxation of the moiré superlattice at twist angles of <2°, and 'topological defect' AA stacking regions, where flat bands are localized, produce a large anomalous local electrochemical enhancement that cannot be accounted for by the elevated local density of states alone.
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35177786What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.