ArticleScience advances2022
Ambient-pressure lignin valorization to high-performance polymers by intensified reductive catalytic deconstruction.
Article in Science advances, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Shaping a Circular Future with Bio-derived Resins in Additive Manufacturing.Accounts of materials research · 2026Article
- Scalable Lignin Monomer Production Via Machine Learning-Guided Reductive Catalytic Fractionation of Lignocellulose.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- PMSE Centennial: Celebration of Success and New Frontiers in Polymer Materials Science and Engineering.ACS macro letters · 2025Article
- Wood-Based Oriented Object Deposition for Programmable Mechanical and 3D Fluidic Control.ACS applied materials & interfaces · 2025Article
- Toward Sustainable Materials: From Lignocellulosic Biomass to High-Performance Polymers.Accounts of materials research · 2025Article
- Investigation on Dynamic and Static Modulus and Creep of Bio-Based Polyurethane-Modified Asphalt Mixture.Polymers · 2025Article
- Article
- Harnessing Atomically Dispersed Cobalt for the Reductive Catalytic Fractionation of Lignocellulose.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Reductive amination cascades in cell-free and resting whole cell formats for valorization of lignin deconstruction products.Biotechnology and bioengineering · 2024Article
- Engineered yeasts and lignocellulosic biomaterials: shaping a new dimension for biorefinery and global bioeconomy.Bioengineered · 2023Review
- Self-Hydrogen Supplied Catalytic Fractionation of Raw Biomass into Lignin-Derived Phenolic Monomers and Cellulose-Rich Pulps.JACS Au · 2023Article
- Photocatalytic Depolymerization of Native Lignin toward Chemically Recyclable Polymer Networks.ACS central science · 2023Article
Corrections and comments
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Authors and funding
11 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Chemocatalytic lignin valorization strategies are critical for a sustainable bioeconomy, as lignin, especially technical lignin, is one of the most available and underutilized aromatic feedstocks. Here, we provide the first report of an intensified reactive distillation–reductive catalytic deconstruction (RD-RCD) process to concurrently deconstruct technical lignins from diverse sources and purify the aromatic products at ambient pressure. We demonstrate the utility of RD-RCD bio-oils in high-performance additive manufacturing via stereolithography 3D printing and highlight its economic advantages over a conventional reductive catalytic fractionation/RCD process. As an example, our RD-RCD reduces the cost of producing a biobased pressure-sensitive adhesive from softwood Kraft lignin by up to 60% in comparison to the high-pressure RCD approach. Last, a facile screening method was developed to predict deconstruction yields using easy-to-obtain thermal decomposition data. This work presents an integrated lignin valorization approach for upgrading existing lignin streams toward the realization of economically viable biorefineries.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.