Evidence map›Paper›PMID 34813290›Full record

ArticleACS applied materials & interfaces2021

Catalyst-Free Synthesis of Lignin Vitrimers with Tunable Mechanical Properties: Circular Polymers and Recoverable Adhesives.

Adrian Moreno, Mohammad Morsali, Mika H Sipponen

Open access · hybridAbstract read
In one paragraph

Article in ACS applied materials & interfaces, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.

0numbers the graph read from it
0cells of the map it votes in
14citing papers in PubMed
7.7field-weighted citation impact, top 1% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

14 citing papers in PubMed, 123 citations in OpenAlex.

  1. Recyclable and bio-based waterborne acetal thermosets and composites.Green chemistry : an international journal and green chemistry resource : GC · 2026
    Article
  2. Article
  3. Article
  4. Article
  5. Article
  6. Review
  7. Review
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  9. Lignin beyond theGreen chemistry : an international journal and green chemistry resource : GC · 2024
    Review
  10. Bio-Based Binder Development for Lithium-Ion Batteries.Materials (Basel, Switzerland) · 2023
    Review
  11. Article
  12. Article
  13. Article
  14. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

3 authors at 1 institution in 1 country.

Adrian MorenoDepartment of Materials and Environmental Chemistry, Stockholm University, Svante Arrhenius Väg 16C, SE-106 91 Stockholm, Sweden.ORCID https://orcid.org/0000-0002-9967-9054
Mohammad MorsaliDepartment of Materials and Environmental Chemistry, Stockholm University, Svante Arrhenius Väg 16C, SE-106 91 Stockholm, Sweden.
Mika H SipponenDepartment of Materials and Environmental Chemistry, Stockholm University, Svante Arrhenius Väg 16C, SE-106 91 Stockholm, Sweden.ORCID https://orcid.org/0000-0001-7747-9310
Stockholm University · SE

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Biobased circular materials are alternatives to fossil-based engineering plastics, but simple and material-efficient synthetic routes are needed for industrial scalability. Here, a series of lignin-based vitrimers built on dynamic acetal covalent networks with a gel content exceeding 95% were successfully prepared in a one-pot, thermally activated, and catalyst-free "click" addition of softwood kraft lignin (SKL) to poly(ethylene glycol) divinyl ether (PDV). The variation of the content of lignin from 28 to 50 wt % was used to demonstrate that the mechanical properties of the vitrimers can be widely tuned in a facile way. The lowest lignin content (28 wt %) showed a tensile strength of 3.3 MPa with 35% elongation at break, while the corresponding values were 50.9 MPa and 1.0% for the vitrimer containing 50 wt % of lignin. These lignin-based vitrimers also exhibited excellent performance as recoverable adhesives for different substrates such as aluminum and wood, with a lap shear test strength of 6.0 and 2.6 MPa, respectively. In addition, recyclability of the vitrimer adhesives showed preservation of the adhesion performance exceeding 90%, indicating a promising potential for their use in sustainable circular materials.

Indexed as

biobased vitrimersligninone-pot synthesisorganic polymersrecyclable adhesives

Identifiers

PMID34813290
PMCPMC8662642
OpenAlexW3217075721

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.