Evidence map›Paper›PMID 34795261›Full record

ArticleNature communications2021

Increasing donor-acceptor spacing for reduced voltage loss in organic solar cells.

Jing Wang, Xudong Jiang, Hongbo Wu, Guitao Feng, Hanyu Wu, Junyu Li, Yuanping Yi, Xunda Feng, Zaifei Ma, Weiwei Li and 2 more

Open access · goldAbstract read
In one paragraph

Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 17 papers.

0numbers the graph read from it
0cells of the map it votes in
17citing papers in PubMed
8.2field-weighted citation impact, top 2% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

17 citing papers in PubMed, 105 citations in OpenAlex.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

12 authors at 4 institutions in 3 countries.

Jing WangState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.ORCID http://orcid.org/0000-0002-3533-1526
Xudong JiangBeijing Advanced Innovation Center for Soft Matter Science and Engineering & State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.
Hongbo WuState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.
Guitao FengBeijing Advanced Innovation Center for Soft Matter Science and Engineering & State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.
Hanyu WuState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.
Junyu LiDSM DMSC R&D Solutions, P.O. Box 18, 6160 MD, Geleen, The Netherlands.
Yuanping YiKey Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, P.R. China.ORCID http://orcid.org/0000-0002-0052-9364
Xunda FengState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.ORCID http://orcid.org/0000-0002-4528-0769
Zaifei MaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.
Weiwei LiBeijing Advanced Innovation Center for Soft Matter Science and Engineering & State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, P. R. China. liweiwei@iccas.ac.cn.ORCID http://orcid.org/0000-0002-7329-4236
Koen VandewalInstituut voor Materiaalonderzoek (IMO-IMOMEC), Hasselt University, Wetenschapspark 1, BE-3590, Diepenbeek, Belgium. koen.vandewal@uhasselt.be.ORCID http://orcid.org/0000-0001-5471-383X
Zheng TangState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China. ztang@dhu.edu.cn.ORCID http://orcid.org/0000-0003-0036-2362
Donghua University · CNChinese Academy of Sciences · CNDSM (Netherlands) · NLHasselt University · BE

Funding

National Natural Science Foundation of China (National Science Foundation of China) 51933001National Natural Science Foundation of China (National Science Foundation of China) 51973031National Natural Science Foundation of China (National Science Foundation of China) 52073016National Natural Science Foundation of China (National Science Foundation of China) 52073056Natural Science Foundation of Shanghai (Natural Science Foundation of Shanghai Municipality) 19ZR1401400
6 · The paper itself

Abstract

The high voltage losses ([Formula: see text]), originating from inevitable electron-phonon coupling in organic materials, limit the power conversion efficiency of organic solar cells to lower values than that of inorganic or perovskite solar cells. In this work, we demonstrate that this [Formula: see text] can in fact be suppressed by controlling the spacing between the donor (D) and the acceptor (A) materials (DA spacing). We show that in typical organic solar cells, the DA spacing is generally too small, being the origin of the too-fast non-radiative decay of charge carriers ([Formula: see text]), and it can be increased by engineering the non-conjugated groups, i.e., alkyl chain spacers in single component DA systems and side chains in high-efficiency bulk-heterojunction systems. Increasing DA spacing allows us to realize significantly reduced [Formula: see text] and improved device voltage. This points out a new research direction for breaking the performance bottleneck of organic solar cells.

Identifiers

PMID34795261
PMCPMC8602729
OpenAlexW3211783724

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.