ArticleAngewandte Chemie (International ed. in English)2022
Unravelling Channel Structure-Diffusivity Relationships in Zeolite ZSM-5 at the Single-Molecule Level.
Article in Angewandte Chemie (International ed. in English), 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Multiscale spatiotemporal heterogeneity of zeolite-catalyzed methanol-to-hydrocarbons reaction.National science review · 2026Review
- Harnessing confinement effect and interpretable machine learning to predict alkane diffusion in zeolite catalysts.Nature communications · 2026Article
- Fluorescent nanoplastics: What steps are needed towards a representative toolkit?Microplastics and nanoplastics · 2026Review
- Exploring the influence of mesoporosity in hard carbon-templated hierarchical SAPO-5 for ethanol dehydration.RSC applied interfaces · 2024Article
- Enhancing sorption kinetics by oriented and single crystalline array-structured ZSM-5 film on monoliths.Nature communications · 2024Article
- Direct probing of single-molecule chemiluminescent reaction dynamics under catalytic conditions in solution.Nature communications · 2023Article
- Emerging analytical methods to characterize zeolite-based materials.National science review · 2022Review
- Classification-based motion analysis of single-molecule trajectories using DiffusionLab.Scientific reports · 2022Article
- Anchoring Effect of Organosilanes on Hierarchical ZSM-5 Zeolite for Catalytic Fast Pyrolysis of Cellulose to Aromatics.ACS omega · 2022Article
- Unravelling Channel Structure-Diffusivity Relationships in Zeolite ZSM-5 at the Single-Molecule Level.Angewandte Chemie (International ed. in English) · 2022Article
Corrections and comments
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Authors and funding
12 authors.
Funding
Abstract
The development of improved zeolite materials for applications in separation and catalysis requires understanding of mass transport. Herein, diffusion of single molecules is tracked in the straight and sinusoidal channels of the industrially relevant ZSM-5 zeolites using a combination of single-molecule localization microscopy and uniformly oriented zeolite thin films. Distinct motion behaviors are observed in zeolite channels with the same geometry, suggesting heterogeneous guest-host interactions. Quantification of the diffusion heterogeneities in the sinusoidal and straight channels suggests that the geometry of zeolite channels dictates the mobility and motion behavior of the guest molecules, resulting in diffusion anisotropy. The study of hierarchical zeolites shows that the addition of secondary pore networks primarily enhances the diffusivity of sinusoidal zeolite channels, and thus alleviating the diffusion limitations of microporous zeolites.
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