ArticleEnvironmental science and pollution research international2022
Effects of Al substitution on sorption of diclofenac to Fe(III) (hydr)oxides: roles of phase transition and sorption mechanisms.
Article in Environmental science and pollution research international, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Fe(III) (hydr)oxides commonly contained many metal impurities such as Al. The incorporation of Al might change the properties of minerals and consequently affect sorption behaviors of pollutants with polar functional groups (e.g., diclofenac (DCF)). In this study, batch experiments and microscale characterization were conducted to investigate the DCF sorption mechanisms to goethite and Al-substituted minerals. Goethite and Al-substituted products (including Al-goethite, Al-goethite-hematite, and Al-hematite) were synthesized with different Al contents (i.e., 0%, 5%, 10%, and 15% (in mol)) by co-precipitation method. Due to difference of ionic radius between Al and Fe and formation of excessive -OH, Al substitution resulted in deviation of cell parameters from the Vegard line. Al substitution caused increasing -OH in Al-goethite and phase transformation caused decreasing -OH in Al-hematite. The total -OH in minerals was positively related to DCF sorption capacity. In the lower initial concentration range (0.4-9 mg/L), the sorption distribution coefficient (K
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