ArticleJournal of the American Chemical Society2021
Dispersity within Brushes Plays a Major Role in Determining Their Interfacial Properties: The Case of Oligoxazoline-Based Graft Polymers.
Article in Journal of the American Chemical Society, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 16 papers.
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Who cites it
16 citing papers in PubMed, 41 citations in OpenAlex.
- Molecular Design of Thermoresponsive Poly(oligoethylene glycol)vinyl Esters for the Generation of Polymer Brush-Based Biointerfaces.ACS polymers Au · 2026Article
- Topological Effects of Bottlebrush Copolymer on Their Assembly at the Water/Air Interface.Langmuir : the ACS journal of surfaces and colloids · 2026Article
- Design, Scalable Synthesis, and Characterization of Poly(Oligourethane Methacrylate)s Bottlebrushes with Discrete, Sequence-Defined, and Stereocontrolled Side-Chains.Macromolecules · 2026Article
- Photo-excited extracellular electron transfer of electroactive microorganism triggers RAFT polymerization.Nature communications · 2025Article
- Anion- and Cation-Specific Response of the Aqueous Conformation of Strong and Weak Polyanionic Brushes.Langmuir : the ACS journal of surfaces and colloids · 2025Article
- Article
- Dispersity-controlled ring-opening polymerization of epoxide.Nature communications · 2025Article
- Orthogonally Functionalizable Redox-Responsive Polymer Brushes: Catch and Release Platform for Proteins and Cells.Journal of the American Chemical Society · 2025Article
- Molecular Design Strategies to Enhance the Electroresponse of Polyelectrolyte Brushes: Effects of Charge Fraction and Chain Length Dispersity.Macromolecules · 2025Article
- Covalent Capture of Nanoparticle-Stabilized Oil Droplets via Acetal Chemistry Using a Hydrophilic Polymer Brush.Langmuir : the ACS journal of surfaces and colloids · 2024Article
- Chromatographic Separation: A Versatile Strategy to Prepare Discrete and Well-Defined Polymer Libraries.Accounts of chemical research · 2024Article
- Controlling primary chain dispersity in network polymers: elucidating the effect of dispersity on degradation.Chemical science · 2023Article
- Design of Microstructure-Engineered Polymers for Energy and Environmental Conservation.JACS Au · 2023Review
- Shaping the Structure and Response of Surface-Grafted Polymer Brushes via the Molecular Weight Distribution.JACS Au · 2023Review
- Xanthate-supported photo-iniferter (XPI)-RAFT polymerization: facile and rapid access to complex macromolecules.Chemical science · 2023Article
- Topologically Precise and Discrete Bottlebrush Polymers: Synthesis, Characterization, and Structure-Property Relationships.JACS Au · 2022Article
Corrections and comments
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Authors and funding
12 authors at 5 institutions in 3 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Many synthetic polymers used to form polymer-brush films feature a main backbone with functional, oligomeric side chains. While the structure of such graft polymers mimics biomacromolecules to an extent, it lacks the monodispersity and structural purity present in nature. Here we demonstrate that side-chain heterogeneity within graft polymers significantly influences hydration and the occurrence of hydrophobic interactions in the subsequently formed brushes and consequently impacts fundamental interfacial properties. This is demonstrated for the case of poly(methacrylate)s (PMAs) presenting oligomeric side chains of different length (
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.