ArticleNature communications2021
A class of organic cages featuring twin cavities.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Kosmotrope-Promoted Proton Hopping in Supramolecular Conductors.Journal of the American Chemical Society · 2026Article
- Self-similar chiral organic molecular cages.Nature communications · 2024Article
- Short hydrogen-bond network confined on COF surfaces enables ultrahigh proton conductivity.Nature communications · 2022Article
- Heterochiral Diastereomer-Discriminative Diphanes That Form Hierarchical Superstructures with Nonlinear Optical Properties.JACS Au · 2022Article
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Authors and funding
14 authors.
Funding
Abstract
A variety of organic cages with different geometries have been developed during the last decade, most of them exhibiting a single cavity. In contrast, the number of organic cages featuring a pair of cavities remains scarce. These structures may pave the way towards novel porous materials with emergent properties and functions.We herein report on rational design of a three-dimensional hexaformyl precursor 1, which exhibits two types of conformers, i.e. Conformer-1 and -2, with different cleft positions and sizes. Aided by molecular dynamics simulations, we select two triamino conformation capturers (denoted CC). Small-sized CC-1 selectively capture Conformer-1 by matching its cleft size, while the large-sized CC-2 is able to match and capture both conformers. This strategy allows the formation of three compounds with twin cavities, which we coin diphane. The self-assembly of diphane units results in superstructures with tunable proton conductivity, which reaches up to 1.37×10
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Registered trials
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