ArticleChemical science2021
Controlled coherent dynamics of [VO(TPP)], a prototype molecular nuclear qudit with an electronic ancilla.
Article in Chemical science, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 16 papers.
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Who cites it
16 citing papers in PubMed, 1 citations in OpenAlex.
- Implementing the Quantum Fourier Transform on a molecular qudit with full refocusing and state tomography.Nature communications · 2026Article
- Oxovanadium(IV) Thiocarboxylate Paddlewheels Containing Ancillary Group 10 Metals: A Comparative Study on Pd and Pt Derivatives.Inorganic chemistry · 2026Article
- Spin Coherence and Electron Spin Distribution of a Silver(II)Inorganic chemistry · 2025Article
- Nutation Spectroscopy of a Weakly Interacting Heterobimetallic Spin System.Chemistry (Weinheim an der Bergstrasse, Germany) · 2025Article
- Room-Temperature Optical Spin Polarization of an Electron Spin Qudit in a Vanadyl-Free Base Porphyrin Dimer.Journal of the American Chemical Society · 2025Article
- Optical Phenomena in Molecule-Based Magnetic Materials.Chemical reviews · 2024Review
- Quantum Mimicry With Inorganic Chemistry.Comments on modern chemistry. Part A, Comments on inorganic chemistry : a journal of critical discussion of the current literature · 2024Article
- Quantum spin coherence and electron spin distribution channels in vanadyl-containing lantern complexes.Inorganic chemistry frontiers · 2023Article
- VdW Mediated Strong Magnetic Exchange Interactions in Chains of Hydrogen-Free Sublimable Molecular Qubits.JACS Au · 2023Article
- The critical role of ultra-low-energy vibrations in the relaxation dynamics of molecular qubits.Nature communications · 2023Article
- An exchange coupledChemical science · 2022Article
- Modelling Conformational Flexibility in a Spectrally Addressable Molecular Multi-Qubit Model System.Angewandte Chemie (International ed. in English) · 2022Article
- Five-Spin Supramolecule for Simulating Quantum Decoherence of Bell States.Journal of the American Chemical Society · 2022Article
- Theoretical Design of Optimal Molecular Qudits for Quantum Error Correction.The journal of physical chemistry letters · 2022Article
- Radiofrequency to Microwave Coherent Manipulation of an Organometallic Electronic Spin Qubit Coupled to a Nuclear Qudit.Inorganic chemistry · 2021Article
- Targeting molecular quantum memory with embedded error correction.Chemical science · 2021Article
Corrections and comments
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Authors and funding
9 authors at 3 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
We show that [VO(TPP)] (vanadyl tetraphenylporphyrinate) is a promising system to implement quantum computation algorithms based on encoding information in multi-level (qudit) units. Indeed, it embeds a nuclear spin 7/2 coupled to an electronic spin 1/2 by hyperfine interaction. This qubit-qudit unit can be exploited to implement quantum error correction and quantum simulation algorithms. Through a combined theoretical and broadband nuclear magnetic resonance study, we demonstrate that the elementary operations of such algorithms can be efficiently implemented on the nuclear spin qudit. Manipulation of the nuclear qudit can be achieved by resonant radio-frequency pulses, thanks to the remarkably long coherence times and the effective quadrupolar coupling induced by the strong hyperfine interaction. This approach may open new perspectives for developing new molecular qubit-qudit systems.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.