ArticleChemSusChem2021
Electroreductive 5-Hydroxymethylfurfural Dimerization on Carbon Electrodes.
Article in ChemSusChem, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
What it found
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Who cites it
10 citing papers in PubMed, 49 citations in OpenAlex.
- Article
- Pairing Electrocatalytic Reduction and Oxidation of Biomass-Derived 5-Hydroxymethylfurfural into Highly Value-Added Chemicals.JACS Au · 2025Article
- Electrochemical Hydrodimerization of Lignocellulose-Derived Carbonyls in Aqueous Electrolytes for Biobased Polymer and Long-chained Synfuel Production: A Review.ChemSusChem · 2025Review
- An alternative to petrochemicals: biomass electrovalorization.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2024Review
- Stability of Bimetallic PtACS materials Au · 2024Article
- Electrocatalytic conversion of biomass-derived furan compounds: mechanisms, catalysts and perspectives.Chemical science · 2024Review
- Hydrogenation versus hydrogenolysis during alkaline electrochemical valorization of 5-hydroxymethylfurfural over oxide-derived Cu-bimetallics.Nature communications · 2023Article
- Recent Progress in Electrochemical Upgrading of Bio-Oil Model Compounds and Bio-Oils to Renewable Fuels and Platform Chemicals.Materials (Basel, Switzerland) · 2023Review
- Insights into the Electrochemical Reduction of 5-Hydroxymethylfurfural at High Current Densities.ChemSusChem · 2022Article
- Article
Corrections and comments
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
Abstract
The electrochemical conversion of biomass-based compounds to fuels and fuel precursors can aid the defossilization of the transportation sector. Herein, the electrohydrodimerization of 5-hydroxymethylfurfural (HMF) to the fuel precursor 5,5'-bis(hydroxymethyl)hydrofuroin (BHH) was investigated on different carbon electrodes. Compared to boron-doped diamond (BDD) electrodes, on glassy carbon (GC) electrodes a less negative HMF reduction onset potential and a switch in product selectivity from BHH to the electrocatalytic hydrogenation product 2,5-di(hydroxymethyl)furan (DHMF) with increasing overpotential was found. On BDD, the electrohydrodimerization was the dominant process independent of the applied potential. An increase in the initial HMF concentration led to suppression of the competing hydrogen evolution reaction and DHMF formation, resulting in higher BHH faradaic efficiencies. In contrast, BHH selectivity decreased with higher initial HMF concentration, which was attributed to increased electrochemically induced HMF degradation. Finally, it was demonstrated that even a simple graphite foil can function as an active HMF electroreduction catalyst.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.