ArticleNature communications2021
A host-guest semibiological photosynthesis system coupling artificial and natural enzymes for solar alcohol splitting.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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6 citing papers in PubMed, 37 citations in OpenAlex.
- All-in-One photo-biocatalysis system for sustainable chemical transformations.Nature communications · 2026Article
- Light-Driven Lithium Extraction from Mixtures of Alkali Cations Using an Azobipyridine Ligand.Journal of the American Chemical Society · 2025Article
- Paramagnetic Cage-Type Co(II) Complexes of Chiral Macrocycles: Enantio- and Size-Selective Binding of Guest Molecules.Inorganic chemistry · 2025Article
- Separation of mercuric ions using 2-thienylbenzimidazole/cucurbit[7]uril/iron-oxide nanoparticles by pH control.Scientific reports · 2023Article
- Electric double layer-mediated polarization field for optimizing photogenerated carrier dynamics and thermodynamics.Nature communications · 2023Article
- Binding of Dual-Function Hybridized MetalJACS Au · 2022Article
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Authors and funding
5 authors at 1 institution in 1 country.
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Abstract
Development of a versatile, sustainable and efficient photosynthesis system that integrates intricate catalytic networks and energy modules at the same location is of considerable future value to energy transformation. In the present study, we develop a coenzyme-mediated supramolecular host-guest semibiological system that combines artificial and enzymatic catalysis for photocatalytic hydrogen evolution from alcohol dehydrogenation. This approach involves modification of the microenvironment of a dithiolene-embedded metal-organic cage to trap an organic dye and NADH molecule simultaneously, serving as a hydrogenase analogue to induce effective proton reduction inside the artificial host. This abiotic photocatalytic system is further embedded into the pocket of the alcohol dehydrogenase to couple enzymatic alcohol dehydrogenation. This host-guest approach allows in situ regeneration of NAD
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