ArticleProceedings of the National Academy of Sciences of the United States of America2021
Inertially enhanced mass transport using 3D-printed porous flow-through electrodes with periodic lattice structures.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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12 citing papers in PubMed, 67 citations in OpenAlex.
- Geometrically periodic architecture for enhanced mass transport in electrocatalysis.Nature communications · 2026Article
- Confinement-enhanced valorization of contaminants in electrified hydrogenation membranes for water purification.Nature communications · 2025Article
- Visualizing nexus of porous architecture and reactive transport in heterogeneous catalysis by deep learning computer vision and transfer learning.Nature communications · 2025Article
- Direct Ink Writing of 3D-Structured All-Carbon Electrodes with High Electrical Conductivity for (Vanadium) Redox Flow Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Understanding the Current Distribution and Mass Transport Properties in 3D-Printed Architected Flow-Through Electrodes.ACS applied engineering materials · 2025Article
- 3D printed optimized electrodes for electrochemical flow reactors.Scientific reports · 2024Article
- Fluid inertia controls mineral precipitation and clogging in pore to network-scale flows.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Development of stochastically reconstructed 3D porous media micromodels using additive manufacturing: numerical and experimental validation.Scientific reports · 2024Article
- Manipulation of Convection Using Infrared Light Emitted from Human Hands.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Unveiling the spatially confined oxidation processes in reactive electrochemical membranes.Nature communications · 2023Article
- Challenges and opportunities in continuous flow processes for electrochemically mediated carbon capture.iScience · 2022Review
- Energy comparison of sequential and integrated CONature communications · 2022Article
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Authors and funding
7 authors at 1 institution in 1 country.
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No grant is acknowledged in the PubMed record.
Abstract
Electrochemical reactors utilizing flow-through electrodes (FTEs) provide an attractive path toward the efficient utilization of electrical energy, but their commercial viability and ultimate adoption hinge on attaining high currents to drive productivity and cost competitiveness. Conventional FTEs composed of random, porous media provide limited opportunity for architectural control and engineering of microscale transport. Alternatively, the design freedom engendered by additively manufacturing FTEs yields additional opportunities to further drive performance via flow engineering. Through experiment and validated continuum computation we analyze the mass transfer in three-dimensional (3D)-printed porous FTEs with periodic lattice structures and show that, in contrast to conventional electrodes, the mesoscopic length scales in 3D-printed electrodes lead to an increase in the mass correlation exponent as inertial flow effects dominate. The inertially enhanced mass transport yields mass transfer coefficients that exceed previously reported 3D-printed FTEs by 10 to 100 times, bringing 3D-printed FTE performance on par with conventional materials.
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