Evidence map›Paper›PMID 34339110›Full record

ArticleChemSusChem2021

Chemo-Biological Upcycling of Poly(ethylene terephthalate) to Multifunctional Coating Materials.

Hee Taek Kim, Mi Hee Ryu, Ye Jean Jung, Sooyoung Lim, Hye Min Song, Jeyoung Park, Sung Yeon Hwang, Hoe-Suk Lee, Young Joo Yeon, Bong Hyun Sung and 4 more

Open access · greenAbstract read
In one paragraph

Article in ChemSusChem, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 19 papers.

0numbers the graph read from it
0cells of the map it votes in
19citing papers in PubMed
3.1field-weighted citation impact, top 7% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

19 citing papers in PubMed, 79 citations in OpenAlex.

  1. Article
  2. Review
  3. Article
  4. Co-consumption for plastics upcycling: A perspective.Metabolic engineering communications · 2025
    Article
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  6. Article
  7. Review
  8. Article
  9. Article
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  12. Review
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  14. Article
  15. Review
  16. Review
  17. Biochemical and structural characterization of an aromatic ring-hydroxylating dioxygenase for terephthalic acid catabolism.Proceedings of the National Academy of Sciences of the United States of America · 2022
    Article
  18. Review
  19. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors at 7 institutions in 2 countries.

Hee Taek KimDepartment of Food Science and Technology, Chungnam National University, Daejeon, 34134 (Republic of, Korea.ORCID http://orcid.org/0000-0002-3941-031X
Mi Hee RyuResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.ORCID http://orcid.org/0000-0002-2538-2100
Ye Jean JungResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.
Sooyoung LimResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.
Hye Min SongDepartment of Chemical Engineering and Materials Science, Graduate Program in System Health Science & Engineering, Ewha Womans University, Seoul, 03760 (Republic of, Korea.
Jeyoung ParkResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.ORCID http://orcid.org/0000-0002-9369-1597
Sung Yeon HwangResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.ORCID http://orcid.org/0000-0002-4618-2132
Hoe-Suk LeeDepartment of Biochemical Engineering, Gangneung-Wonju National University, Gangneung-si, Gangwon-do, 25457 (Republic of, Korea.ORCID http://orcid.org/0000-0001-9237-607X
Young Joo YeonDepartment of Biochemical Engineering, Gangneung-Wonju National University, Gangneung-si, Gangwon-do, 25457 (Republic of, Korea.ORCID http://orcid.org/0000-0003-1400-8014
Bong Hyun SungSynthetic Biology and Bioengineering Research Center, Korea Research Institute of Bioscience and Biotechnology, Daejeon, 34141 (Republic of, Korea.ORCID http://orcid.org/0000-0002-8992-1118
Uwe T BornscheuerDepartment of Biotechnology & Enzyme Catalysis, Institute of Biochemistry, University of Greifswald, 17487, Greifswald, Germany.ORCID http://orcid.org/0000-0003-0685-2696
Si Jae ParkDepartment of Chemical Engineering and Materials Science, Graduate Program in System Health Science & Engineering, Ewha Womans University, Seoul, 03760 (Republic of, Korea.ORCID http://orcid.org/0000-0001-9735-4582
Jeong Chan JooResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.ORCID http://orcid.org/0000-0001-5393-7057
Dongyeop X OhResearch Center for Bio-based Chemicals, Korea Research Institute of Chemical Technology, Daejeon, 34114 & Ulsan 44429 (Republic of, Korea.ORCID http://orcid.org/0000-0003-3665-405X
Korea Research Institute of Chemical Technology · KREwha Womans University · KRGangneung–Wonju National University · KRChungnam National University · KRKorea Research Institute of Bioscience and Biotechnology · KRThe Catholic University of Korea Bucheon St. Mary's Hospital · KRUniversitätsmedizin Greifswald · DE

Funding

Ministry of Science NRF-2020R1A5A1019631Ministry of Science NRF-2020R1C1C1005719Ministry of Science NRF-2021R1A2C2011669
6 · The paper itself

Abstract

Chemo-biological upcycling of poly(ethylene terephthalate) (PET) developed in this study includes the following key steps: chemo-enzymatic PET depolymerization, biotransformation of terephthalic acid (TPA) into catechol, and its application as a coating agent. Monomeric units were first produced through PET glycolysis into bis(2-hydroxyethyl) terephthalate (BHET), mono(2-hydroxyethyl) terephthalate (MHET), and PET oligomers, and enzymatic hydrolysis of these glycolyzed products using Bacillus subtilis esterase (Bs2Est). Bs2Est efficiently hydrolyzed glycolyzed products into TPA as a key enzyme for chemo-enzymatic depolymerization. Furthermore, catechol solution produced from TPA via a whole-cell biotransformation (Escherichia coli) could be directly used for functional coating on various substrates after simple cell removal from the culture medium without further purification and water-evaporation. This work demonstrates a proof-of-concept of a PET upcycling strategy via a combination of chemo-biological conversion of PET waste into multifunctional coating materials.

Indexed as

Bacillus subtilisBiotransformationCatecholsCoated Materials, BiocompatibleEscherichia coliEsterasesGlycolysisHydrolysisModels, MolecularPhthalic AcidsPolyethylene TerephthalatesProtein ConformationcatecholCatecholsCoated Materials, BiocompatibleEsterasesPhthalic AcidsPolyethylene Terephthalatesterephthalic acidbiocatalysiscatecholesterasepoly(ethylene terephthalate)upcycling

Identifiers

PMID34339110
PMCPMC8519047
OpenAlexW3191669101

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.