ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2020
From SERS to TERS and Beyond: Molecules as Probes of Nanoscopic Optical Fields.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Investigating the Role of Plasmonics in Electrospun Fibers by Combined Photothermal Heterodyne Imaging and Raman Measurements.The journal of physical chemistry. C, Nanomaterials and interfaces · 2024Article
- Role of Plasmonic Antenna in Hot Carrier-Driven Reactions on Bimetallic Nanostructures.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Mechanism for plasmon-generated solvated electrons.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Multipolar Raman Scattering vs Interfacial Nanochemistry: Case of 4-Mercaptopyridine on Gold.Journal of the American Chemical Society · 2022Article
- Spatially-Localized Functionalization on Nanostructured Surfaces for Enhanced Plasmonic Sensing Efficacy.Nanomaterials (Basel, Switzerland) · 2022Article
- SERS/TERS Characterization of New Potential Therapeutics: The Influence of Positional Isomerism, Interface Type, Oxidation State of Copper, and Incubation Time on Adsorption on the Surface of Copper(I) and (II) Oxide Nanoparticles.Journal of medicinal chemistry · 2022Article
- Spectrally Resolved Surface-Enhanced Raman Scattering Imaging Reveals Plasmon-Mediated Chemical Transformations.ACS nanoscience Au · 2021Article
Corrections and comments
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Authors and funding
2 authors.
Funding
Abstract
A detailed understanding of the interaction between molecules and plasmonic nanostructures is important for several exciting developments in (bio)molecular sensing and imaging, catalysis, as well as energy conversion. While much of the focus has been on the nanostructures that generate enhanced and nano-confined optical fields, we herein highlight recent work from our groups that uses the molecular response in surface and tip enhanced Raman scattering (SERS and TERS, respectively) to investigate different aspects of the local fields. TERS provides access to ultra-confined volumes, and as a result can further explore and explain ensemble-averaged SERS measurements. Exciting and distinct molecular behaviors are observed in the quantum limit of plasmons, including molecular charging, chemical conversion, and optical rectification. Evidence of multipolar Raman scattering from molecules additionally provides insights into the inhomogeneous electric fields that drive SERS and TERS and their spatial and temporal gradients. The time scales of these processes show evidence of cooperative nanoscale phenomena that altogether contribute to SERS and TERS.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.