ArticleChemistry (Weinheim an der Bergstrasse, Germany)2021
Binding Sites, Vibrations and Spin-Lattice Relaxation Times in Europium(II)-Based Metallofullerene Spin Qubits.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed, 21 citations in OpenAlex.
- Orientationally Resolved Electron-Spin Relaxation and Coherence in Fullerene-Encapsulated Rare-Earth Dimers with a Single-Electron Metal-Metal Bond.Journal of the American Chemical Society · 2026Article
- Exploring a New Family of (Phosphinochalcogenoyl)Europocenes for Magneto-Optical Thermometry.Angewandte Chemie (International ed. in English) · 2025Article
- Controlling Magnetic Anisotropy of Endohedral Lanthanide Ions by Carbene Addition: Paramagnetic NMR, Lanthanide Luminescence, and Single-Molecule Magnetism in Adamantylidene Adducts of MScJournal of the American Chemical Society · 2025Article
- Chemical Origins of Optically Addressable Spin States in EuACS materials Au · 2025Article
- CaY@CJournal of the American Chemical Society · 2024Article
- Computational design of magnetic molecules and their environment using quantum chemistry, machine learning and multiscale simulations.Nature reviews. Chemistry · 2022Review
- Binding Sites, Vibrations and Spin-Lattice Relaxation Times in Europium(II)-Based Metallofullerene Spin Qubits.Chemistry (Weinheim an der Bergstrasse, Germany) · 2021Article
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Authors and funding
9 authors at 2 institutions in 2 countries.
Funding
Abstract
To design molecular spin qubits with enhanced quantum coherence, a control of the coupling between the local vibrations and the spin states is crucial, which could be realized in principle by engineering molecular structures via coordination chemistry. To this end, understanding the underlying structural factors that govern the spin relaxation is a central topic. Here, we report the investigation of the spin dynamics in a series of chemically designed europium(II)-based endohedral metallofullerenes (EMFs). By introducing a unique structural difference, i. e. metal-cage binding site, while keeping other molecular parameters constant between different complexes, these manifest the key role of the three low-energy metal-displacing vibrations in mediating the spin-lattice relaxation times (T
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