ArticleNature communications2021
Quantitative 3D real-space analysis of Laves phase supraparticles.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Cooperative and collective quantum light emission from perovskite superball superstructures.Science advances · 2026Article
- Discovery of confined two-dimensional Laves tiling in a magnesium alloy.Nature communications · 2026Article
- A Robust Synthesis of Fluorosurfactants with Tunable Functionalities via a Two-Step Reaction.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Pushing the Frontiers: Artificial Intelligence (AI)-Guided Programmable Concepts in Binary Self-Assembly of Colloidal Nanoparticles.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Review
- Quantitative 3D structural analysis of small colloidal assemblies under native conditions by liquid-cell fast electron tomography.Nature communications · 2024Article
- Structural diversity in three-dimensional self-assembly of nanoplatelets by spherical confinement.Nature communications · 2022Article
- Efficient event-driven simulations of hard spheres.The European physical journal. E, Soft matter · 2022Article
Corrections and comments
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Authors and funding
10 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Assembling binary mixtures of nanoparticles into crystals, gives rise to collective properties depending on the crystal structure and the individual properties of both species. However, quantitative 3D real-space analysis of binary colloidal crystals with a thickness of more than 10 layers of particles has rarely been performed. Here we demonstrate that an excess of one species in the binary nanoparticle mixture suppresses the formation of icosahedral order in the self-assembly in droplets, allowing the study of bulk-like binary crystal structures with a spherical morphology also called supraparticles. As example of the approach, we show single-particle level analysis of over 50 layers of Laves phase binary crystals of hard-sphere-like nanoparticles using electron tomography. We observe a crystalline lattice composed of a random mixture of the Laves phases. The number ratio of the binary species in the crystal lattice matches that of a perfect Laves crystal. Our methodology can be applied to study the structure of a broad range of binary crystals, giving insights into the structure formation mechanisms and structure-property relations of nanomaterials.
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