ArticleChemical science2021
High-resolution imaging of catalytic activity of a single graphene sheet using electrochemiluminescence microscopy.
Article in Chemical science, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed, 55 citations in OpenAlex.
- Electrochemiluminescence and Photoinduced Electrochemiluminescence Probing of Energy Conversion Catalysis.Chemical & biomedical imaging · 2026Review
- Electrochemiluminescence Imaging for In Situ Electrocatalysis Characterization: Recent Progress and Mechanistic Insights.Chemical & biomedical imaging · 2026Review
- Breathing Laser-Spectral Mapping of Cavity-Enhanced Redox Reactions with Subcellular Resolution.ACS nano · 2025Article
- Photo-crosslinking of doped magic-sized nanoclusters for the construction of enhanced electrochemiluminescence biosensors.Chemical science · 2025Article
- A mini-review on the research progress and application of nanomaterials in electrochemiluminescent sensors in the detection of water environmental pollutants.Mikrochimica acta · 2025Review
- Enhanced Electrochemiluminescence at the Gas/Liquid Interface of Bubbles Propelled into Solution.Journal of the American Chemical Society · 2024Article
- Nanoscale Luminescence Imaging/Detection of Single Particles: State-of-the-Art and Future Prospects.ACS measurement science au · 2024Review
- Site-selective heat boosting electrochemiluminescence for single cell imaging.Chemical science · 2023Article
- A Close Look at Mechanism, Application, and Opportunities of Electrochemiluminescence Microscopy.Chemical & biomedical imaging · 2023Review
- Newly Developed Electrochemiluminescence Based on Bipolar Electrochemistry for Multiplex Biosensing Applications: A Consolidated Review.Biosensors · 2023Review
- Highly Sensitive Detection of the Insecticide Azamethiphos by Tris(2,2'-bipyridine)ruthenium(II) Electrogenerated Chemiluminescence.Sensors (Basel, Switzerland) · 2022Article
- A Guide Inside Electrochemiluminescent Microscopy Mechanisms for Analytical Performance Improvement.Analytical chemistry · 2022Article
Corrections and comments
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Authors and funding
3 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Here, the electrocatalytic activity of a single graphene sheet is mapped using electrochemiluminescence (ECL) microscopy with a nanometer resolution. The achievement of this high-spatial imaging relies on the varied adsorption of hydrogen peroxide at different sites on the graphene surface, leading to unsynchronized ECL emission. By shortening the exposure time to 0.2 ms, scattered ECL spots are observed in the ECL image that are not overlaid with the spots in the consecutive images. Accordingly, after stacking all the images into a graph, the ECL intensity of each pixel could be used to reflect the electrocatalytic features of the graphene surface with a resolution of 400 nm. This novel ECL method efficiently avoids the long-standing problem of classic ECL microscopy regarding the overlap of ECL emissions from adjacent regions and enables the nanometer spatial resolution of ECL microscopy for the first time.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.