ArticleNature communications2021
Chiral high-harmonic generation and spectroscopy on solid surfaces using polarization-tailored strong fields.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Pulse-Duration-Sensitive High Harmonics and Attosecond Locally Chiral Near Fields from a Chiral Topological Weyl Semimetal.Nano letters · 2026Article
- Non-cascade random walks in solid-state high harmonic generation.Nature communications · 2026Article
- High power, dual SWIR-MIR OPCPA source for high-order harmonics generation.Scientific reports · 2025Article
- Incongruous Harmonics of Vibrating Solid-Solid Interface.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- High harmonic spectroscopy reveals anisotropy of the charge-density-wave phase transition in TiSeCommunications materials · 2025Article
- Valleytronics in bulk MoSNature · 2024Article
- Intrinsic dichroism in amorphous and crystalline solids with helical light.Nature communications · 2024Article
- Selection rules in symmetry-broken systems by symmetries in synthetic dimensions.Nature communications · 2022Article
Corrections and comments
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Authors and funding
7 authors.
Funding
Abstract
Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media offers unprecedented possibilities to control high-harmonic generation using modified targets or tailored excitation fields. Here we merge these important points and demonstrate circularly-polarized high-harmonic generation with polarization-matched excitation fields for spectroscopy of chiral electronic properties at surfaces. The sensitivity of our approach is demonstrated for structural helicity and termination-mediated ferromagnetic order at the surface of silicon-dioxide and magnesium oxide, respectively. Circularly polarized radiation emanating from a solid sample now allows to add basic symmetry properties as chirality to the arsenal of strong-field spectroscopy in solids. Together with its inherent temporal (femtosecond) resolution and non-resonant broadband spectrum, the polarization control of high harmonics from condensed matter can illuminate ultrafast and strong field dynamics of surfaces, buried layers or thin films.
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Registered trials
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