ReviewAngewandte Chemie (International ed. in English)2021
Synthesis of N-Heterocycles via Oxidant-Free Dehydrocyclization of Alcohols Using Heterogeneous Catalysts.
Review in Angewandte Chemie (International ed. in English), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Synthesis of Azaisoindolinones by Heterogeneous Catalyzed Regioselective Hydrodeoxygenation ofACS sustainable chemistry & engineering · 2025Article
- Heterogeneous Mn@CeOACS omega · 2025Article
- Oxygen Vacancies in β-MoOResearch (Washington, D.C.) · 2025Article
- Multicomponent synthesisRSC advances · 2024Article
- Cobalt nanoparticle-catalysedGreen chemistry : an international journal and green chemistry resource : GC · 2024Article
- Article
- N, S Co-Coordinated Zinc Single-Atom Catalysts for N-Alkylation of Aromatic Amines with Alcohols: The Role of S-Doping in the Reaction.Nanomaterials (Basel, Switzerland) · 2023Article
- Synthesis and characterization of thiophene-derived palladium(ii) complex immobilized on FSM-16 and its application in the novel synthesis of 7-(aryl)-7,12-dihydro-6RSC advances · 2022Article
- Recent Advances in Carbon-Based Iron Catalysts for Organic Synthesis.Nanomaterials (Basel, Switzerland) · 2022Review
- Catalytic oxidative dehydrogenation of N-heterocycles with nitrogen/phosphorus co-doped porous carbon materials.Chemical science · 2022Article
- Efficient iron single-atom catalysts for selective ammoxidation of alcohols to nitriles.Nature communications · 2022Article
- Synthesis of N-Heterocycles via Oxidant-Free Dehydrocyclization of Alcohols Using Heterogeneous Catalysts.Angewandte Chemie (International ed. in English) · 2021Review
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5 authors.
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Abstract
N-Heterocycles, such as pyrroles, pyrimidines, quinazolines, and quinoxalines, are important building blocks for organic chemistry and the fine-chemical industry. For their synthesis, catalytic borrowing hydrogen and acceptorless dehydrogenative coupling reactions of alcohols as sustainable reagents have received significant attention in recent years. To overcome the problems of product separation and catalyst reusability, several metal-based heterogeneous catalysts have been reported to achieve these transformations with good yields and selectivity. In this Minireview, we summarize recent developments using both noble and non-noble metal-based heterogeneous catalysts to synthesize N-heterocycles from alcohols and N-nucleophiles via acceptorless dehydrogenation or borrowing hydrogen methodologies. Furthermore, this Minireview introduces strategies for the preparation and functionalization of the corresponding heterogeneous catalysts, discusses the reaction mechanisms and the roles of metal electronic states, and the influence of support Lewis acid-base properties on these reactions.
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