ArticleNature communications2021
Manifestations of metastable criticality in the long-range structure of model water glasses.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed, 27 citations in OpenAlex.
- Unravelling Water Anomalies Using a Percolation Approach.ACS omega · 2026Article
- Computational investigation of water glasses using machine-learning potentials.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Medium-density amorphous ice unveils shear rate as a new dimension in water's phase diagram.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Liquid-liquid transition and ice crystallization in a machine-learned coarse-grained water model.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- A continuum of amorphous ices between low-density and high-density amorphous ice.Communications chemistry · 2024Article
- Article
- Evidence of a liquid-liquid phase transition in H[Formula: see text]O and D[Formula: see text]O from path-integral molecular dynamics simulations.Scientific reports · 2022Article
- Percolation transitions in compressed SiONature · 2021Article
- The role of high-density and low-density amorphous ice on biomolecules at cryogenic temperatures: a case study with polyalanine.Physical chemistry chemical physics : PCCP · 2021Article
- Linking amorphous ice and supercooled liquid water.Proceedings of the National Academy of Sciences of the United States of America · 2021Article
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
Abstract
Much attention has been devoted to water's metastable phase behavior, including polyamorphism (multiple amorphous solid phases), and the hypothesized liquid-liquid transition and associated critical point. However, the possible relationship between these phenomena remains incompletely understood. Using molecular dynamics simulations of the realistic TIP4P/2005 model, we found a striking signature of the liquid-liquid critical point in the structure of water glasses, manifested as a pronounced increase in long-range density fluctuations at pressures proximate to the critical pressure. By contrast, these signatures were absent in glasses of two model systems that lack a critical point. We also characterized the departure from equilibrium upon vitrification via the non-equilibrium index; water-like systems exhibited a strong pressure dependence in this metric, whereas simple liquids did not. These results reflect a surprising relationship between the metastable equilibrium phenomenon of liquid-liquid criticality and the non-equilibrium structure of glassy water, with implications for our understanding of water phase behavior and glass physics. Our calculations suggest a possible experimental route to probing the existence of the liquid-liquid transition in water and other fluids.
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