ArticleChemical science2020
Controlled synthesis of organic two-dimensional nanostructures
Article in Chemical science, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Crystallization-driven two-dimensional assemblies from a phenothiazine-conjugated poly(l-lactide): redox-responsive tunable emission, white-light harvesting and surface-enabled nanoparticle decoration.Chemical science · 2025Article
- Expanding the Scope of Metastable Species in Hydrogen Bonding-Directed Supramolecular Polymerization.Angewandte Chemie (International ed. in English) · 2022Article
- Bottom-up supramolecular assembly in two dimensions.Chemical science · 2022Review
- Hierarchical self-assembly of aromatic peptide conjugates into supramolecular polymers: it takes two to tango.Chemical science · 2022Review
- Substrate induced generation of transient self-assembled catalytic systems.Chemical science · 2021Review
- Tubular supramolecular alternating copolymers fabricated by cyclic peptide-polymer conjugates.Chemical science · 2021Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The bottom-up approach of supramolecular polymerization is an effective synthetic method for functional organic nanostructures. However, the uncontrolled growth and polydisperse structural outcome often lead to low functional efficiency. Thus, precise control over the structural characteristics of supramolecular polymers is the current scientific hurdle. Research so far has tended to focus on systems with inherent kinetic control by the presence of metastable state monomers either through conformational molecular design or by exploring pathway complexity. The need of the hour is to create generic strategies for dormant states of monomers that can be extended to different molecules and various structural organizations and dimensions. Here we venture to demonstrate chemical reaction-driven cooperative supramolecular polymerization as an alternative strategy for the controlled synthesis of organic two-dimensional nanostructures. In our approach, the dynamic imine bond is exploited to convert a non-assembling dormant monomer to an activated amphiphilic structure in a kinetically controlled manner. The chemical reaction governed retarded nucleation-elongation growth provides control over dispersity and size.
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Registered trials
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