Evidence map›Paper›PMID 34094056›Full record

ArticleChemical science2020

Site-specific growth of MOF-on-MOF heterostructures with controllable nano-architectures: beyond the combination of MOF analogues.

Chao Liu, Lina Lin, Qiang Sun, Jing Wang, Rong Huang, Wenyi Chen, Shumin Li, Jingjing Wan, Jin Zou, Chengzhong Yu

Open access · diamondAbstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Chemical science, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.

0numbers the graph read from it
0cells of the map it votes in
11citing papers in PubMed
6.2field-weighted citation impact, top 3% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

11 citing papers in PubMed, 154 citations in OpenAlex.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

10 authors at 2 institutions in 4 countries.

Chao LiuSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.
Lina LinKey Laboratory of Polar Materials and Devices (MOE), Department of Electronics, East China Normal University Shanghai 200241 P. R. China.
Qiang SunMaterials Engineering, University of Queensland Brisbane Queensland 4072 Australia j.zou@uq.edu.au.ORCID https://orcid.org/0000-0001-5328-7605
Jing WangSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.
Rong HuangKey Laboratory of Polar Materials and Devices (MOE), Department of Electronics, East China Normal University Shanghai 200241 P. R. China.
Wenyi ChenSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.
Shumin LiSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.
Jingjing WanSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.
Jin ZouMaterials Engineering, University of Queensland Brisbane Queensland 4072 Australia j.zou@uq.edu.au.ORCID https://orcid.org/0000-0001-9435-8043
Chengzhong YuSchool of Chemistry and Molecular Engineering, East China Normal University Shanghai 200241 P. R. China jjwan@chem.ecnu.edu.cn czyu@chem.ecnu.edu.cn.ORCID https://orcid.org/0000-0003-3707-0785
East China Normal University · CNThe University of Queensland · AU

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The integration of different metal-organic frameworks (MOFs) into one system has led to the recent combinatorial innovation of various MOF-on-MOF hybrids; however control over their site-specific growth beyond MOF analogues remains challenging. In this work, a site-specific epitaxial-growth strategy is developed to synthesize MOF-on-MOF heterostructures comprised of two MOFs with totally different compositions. A guest MOF (ZIF-8) is epitaxially grown on the specific {110} facets of a host MOF (MIL-125). Moreover, the position of ZIF-8 growth on MIL-125 is also selectable by using MIL-125 hosts with {110} facets exposed on either the corner or side surface. Consequently, two MIL-125@ZIF-8 heterostructures with elaborately designed different architectures are synthesized. Benefiting from the high adsorption capacity of ZIF-8 and the photocatalytic activity of MIL-125, the MIL-125@ZIF-8 heterostructures demonstrate synergistically enhanced photocatalytic performance compared to single MOF subunits. Moreover, the corner growth leads to higher activity than the side growth of the MIL-125@ZIF-8 heterostructures. Our contribution paves the way for the rational design of composite MOFs with tunable compositions and nanostructures using the crystal engineering approach.

Identifiers

PMID34094056
PMCPMC8152623
OpenAlexW3010133597

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.