ArticleACS applied polymer materials2020
Combined Dynamic Network and Filler Interface Approach for Improved Adhesion and Toughness in Pressure-Sensitive Adhesives.
Article in ACS applied polymer materials, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Robust and Reversible Supramolecular Adhesive via Dynamic Covalent Bond Crosslinking-Induced Assembly of Metal-Coordinated Nanoparticles.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- High-performance reversible adhesive from PET waste for underwater, structural, and pressure-sensitive applications.Science advances · 2025Article
- Taking dynamic covalent chemistry out of the lab and into reprocessable industrial thermosets.Nature reviews. Chemistry · 2025Review
- Integrating Bioinspired Natural Adhesion Mechanisms into Modified Polyacrylate Latex Pressure-Sensitive Adhesives.Polymers · 2024Article
- Re-Assemblable, Recyclable, and Self-Healing Epoxy Resin Adhesive Based on Dynamic Boronic Esters.Polymers · 2023Article
- Bioinspired nucleobase-containing polyelectrolytes as robust and tunable adhesives by balancing the adhesive and cohesive properties.Chemical science · 2023Article
- Study of Applying Naturally Occurring Mineral Materials for Silicone Pressure-Sensitive Adhesives.Materials (Basel, Switzerland) · 2023Article
- Design of tough adhesive from commodity thermoplastics through dynamic crosslinking.Science advances · 2021Article
- Vitrimers: directing chemical reactivity to control material properties.Chemical science · 2020Review
Corrections and comments
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Authors and funding
3 authors.
Funding
Abstract
Of importance for adhesive materials, particularly pressure-sensitive adhesive (PSA) systems, is the ability to increase bulk toughness without reduction of adhesion. Previous approaches for increasing PSA durability sacrifice permanent cross-linking or adhesive potential, limiting performance. In this work, covalent adaptable networks (CANs) derived from thiol-thioester exchange (TTE) are utilized as a basis for adhesive films. Tensile and single-lap shear tests were conducted for adhesive materials containing no filler, 15 wt % nanoparticles functionalized with thioester-containing acrylate, or 15 wt % nanoparticles functionalized with nonthioester-containing acrylate. Additionally, fatigue experiments were conducted on unfilled adhesives. Results indicate that TTE improves toughness, adhesion, and fatigue in unfilled materials. Filled adhesives with activated TTE showed a nearly fourfold increase in adhesion with slightly reduced toughness compared to uncatalyzed filled specimens. This work has implications in many industries, from biomedical to automotive, as toughness and fatigue resistance are important considerations for adhesive applications.
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