ArticleStructural dynamics (Melville, N.Y.)2021
Capturing fingerprints of conical intersection: Complementary information of non-adiabatic dynamics from linear x-ray probes.
Article in Structural dynamics (Melville, N.Y.), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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Who cites it
3 citing papers in PubMed, 9 citations in OpenAlex.
- Raman Spectroscopy of Conical Intersections Using Entangled Photons.The journal of physical chemistry letters · 2024Article
- Time-resolved X-ray and XUV based spectroscopic methods for nonadiabatic processes in photochemistry.Chemical communications (Cambridge, England) · 2022Review
- Time-Resolved Photoelectron Spectroscopy of Conical Intersections with Attosecond Pulse Trains.The journal of physical chemistry letters · 2021Article
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Authors and funding
3 authors at 1 institution in 1 country.
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Abstract
Many recent experimental ultrafast spectroscopy studies have hinted at non-adiabatic dynamics indicating the existence of conical intersections, but their direct observation remains a challenge. The rapid change of the energy gap between the electronic states complicated their observation by requiring bandwidths of several electron volts. In this manuscript, we propose to use the combined information of different x-ray pump-probe techniques to identify the conical intersection. We theoretically study the conical intersection in pyrrole using transient x-ray absorption, time-resolved x-ray spontaneous emission, and linear off-resonant Raman spectroscopy to gather evidence of the curve crossing.
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