ArticleAngewandte Chemie (International ed. in English)2021
FRET-Integrated Polymer Brushes for Spatially Resolved Sensing of Changes in Polymer Conformation.
Article in Angewandte Chemie (International ed. in English), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 24 papers.
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Who cites it
24 citing papers in PubMed.
- Stimuli-Responsive Hierarchical Structuring Controls Survival and Programs Hydrogelation of Supramolecular Metallofibers.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Characterization of swelling gradients and evaporation dynamics in polymer brushes using high-resolution colorimetry.The European physical journal. E, Soft matter · 2026Article
- Unveiling the fluorescence lifetime changes of a solvatochromic aurone probe dye upon wetting in an emissive polymer brush matrix by deconvolution of TCSPC data.The European physical journal. E, Soft matter · 2026Article
- Nano-visualization of hydrogel dynamicsChemical science · 2026Article
- Rational design of pigment-polymer antenna complexes.Chemical science · 2026Article
- Exploring Scent Distinction with Polymer Brush Arrays.ACS applied polymer materials · 2025Article
- Machine Learning in Polymer Research.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Molecular Design Strategies to Enhance the Electroresponse of Polyelectrolyte Brushes: Effects of Charge Fraction and Chain Length Dispersity.Macromolecules · 2025Article
- Capturing Conformational Transitions of Fluorescently-Coupled Polyelectrolyte Brushes with High Spatiotemporal Resolution.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- On the Road to Circular Polymer Brushes: Challenges and Prospects.Langmuir : the ACS journal of surfaces and colloids · 2024Review
- PNIPAM Brushes in Colloidal Photonic Crystals Enable Ex Situ Ethanol Vapor Sensing.ACS applied polymer materials · 2024Article
- PolyNC: a natural and chemical language model for the prediction of unified polymer properties.Chemical science · 2024Article
- Navigating the Expansive Landscapes of Soft Materials: A User Guide for High-Throughput Workflows.ACS polymers Au · 2023Review
- Integrated FRET Polymers Spatially Reveal Micro- to Nanostructure and Irregularities in Electrospun Microfibers.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Fluorescence-readout as a powerful macromolecular characterisation tool.Chemical science · 2023Review
- Polyester Brush Coatings for Circularity: Grafting, Degradation, and Repeated Growth.Macromolecules · 2023Article
- Scalable Air-Tolerant μL-Volume Synthesis of Thick Poly(SPMA) Brushes Using SI-ARGET-ATRP.ACS applied polymer materials · 2023Article
- Swelling-Activated, Soft Mechanochemistry in Polymer Materials.Langmuir : the ACS journal of surfaces and colloids · 2023Review
- Article
- Enhanced vapor sorption in block and random copolymer brushes.Soft matter · 2022Article
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Polymer brush surfaces that alter their physical properties in response to chemical stimuli have the capacity to be used as new surface-based sensing materials. For such surfaces, detecting the polymer conformation is key to their sensing capabilities. Herein, we report on FRET-integrated ultrathin (<70 nm) polymer brush surfaces that exhibit stimuli-dependent FRET with changing brush conformation. Poly(N-isopropylacrylamide) polymers were chosen due their exceptional sensitivity to liquid mixture compositions and their ability to be assembled into well-defined polymer brushes. The brush transitions were used to optically sense changes in liquid mixture compositions with high spatial resolution (tens of micrometers), where the FRET coupling allowed for noninvasive observation of brush transitions around complex interfaces with real-time sensing of the liquid environment. Our methods have the potential to be leveraged towards greater surface-based sensing capabilities at intricate interfaces.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.