ArticleNature communications2021
Oriented arrangement of simple monomers enabled by confinement: towards living supramolecular polymerization.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
What it found
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Who cites it
4 citing papers in PubMed, 26 citations in OpenAlex.
- Controlled assembly of two-dimensional porphyrin heterostructures toward directed energy transfer and charge separation.Nature communications · 2026Article
- Confinement-Induced Metastable Supramolecular Assembly: Dynamic Built-in Electric Field Driving Deep Mineralization of Organic Pollutants.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Instability-induced crystal self-assembly in film-substrate system for the construction of large-area micro- and nano-chiral structures.Nature communications · 2025Article
- Therapeutic Supramolecular Polymers: Designs and Applications.Progress in polymer science · 2024Article
Corrections and comments
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The living supramolecular polymerization technique provides an exciting research avenue. However, in comparison with the thermodynamic spontaneous nucleation, using simple monomers to realize living supramolecular polymerization is hardly possible from an energy principle. This is because the activation barrier of kinetically trapped simple monomer (nucleation step) is insufficiently high to control the kinetics of subsequent elongation. Here, with the benefit of the confinement from the layered double hydroxide (LDH) nanomaterial, various simple monomers, (such as benzene, naphthalene and pyrene derivatives) successfully form living supramolecular polymer (LSP) with length control and narrow dispersity. The degree of polymerization can reach ~6000. Kinetics studies reveal LDH overcomes a huge energy barrier to inhibit undesired spontaneous nucleation of monomers and disassembly of metastable states. The universality of this strategy will usher exploration into other multifunctional molecules and promote the development of functional LSP.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.