ArticleScience advances2021
Nonlinear infrared polaritonic interaction between cavities mediated by molecular vibrations at ultrafast time scale.
Article in Science advances, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Reservoir Dynamics in Vibrational Polaritons Revealed by Detuning-Dependent Ultrafast Spectroscopy.The journal of physical chemistry letters · 2026Article
- Direct Readout of Excited-State Lifetimes in Chlorin Chromophores under Electronic Strong Coupling.Journal of the American Chemical Society · 2026Article
- Phase-Resolved Two-Dimensional Infrared Spectroscopy of Solution-Phase Vibrational Polaritons on Gold Antenna Meta-Surfaces.The journal of physical chemistry letters · 2026Article
- Excited State Dynamics of COJournal of the American Chemical Society · 2025Article
- Spatially Resolved Near Field Spectroscopy of Vibrational Polaritons at the Small N Limit.ACS photonics · 2024Article
- Ultrafast Spectroscopy under Vibrational Strong Coupling in Diphenylphosphoryl Azide.The journal of physical chemistry. A · 2024Article
- Molecular Polaritons for Chemistry, Photonics and Quantum Technologies.Chemical reviews · 2024Review
- Molecular Vibrational Polariton Dynamics: What Can Polaritons Do?Accounts of chemical research · 2023Article
- Polaritons in modified Fabry-Perot cavities and entanglement.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Enabling multiple intercavity polariton coherences by adding quantum confinement to cavity molecular polaritons.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Analysis of a q-deformed hyperbolic short laser pulse in a multi-level atomic system.Scientific reports · 2022Article
- Cavity catalysis: modifying linear free-energy relationship under cooperative vibrational strong coupling.Chemical science · 2021Article
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Realizing nonlinear interactions between spatially separated particles can advance molecular science and technology, including remote catalysis of chemical reactions, ultrafast processing of information in infrared (IR) photonic circuitry, and advanced platforms for quantum simulations with increased complexity. Here, we achieved nonlinear interactions at ultrafast time scale between polaritons contained in spatially adjacent cavities in the mid-IR regime, altering polaritons in one cavity by pumping polaritons in an adjacent one. This was done by strong coupling molecular vibrational modes with photon modes, a process that combines characteristics of both photon delocalization and molecular nonlinearity. The dual photon/molecule character of polaritons enables delocalized nonlinearity-a property that neither molecular nor cavity mode would have alone.
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Registered trials
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