ArticleNanomaterials (Basel, Switzerland)2021
Tunable Synthesis of Predominant Semi-Ionic and Covalent Fluorine Bonding States on a Graphene Surface.
Article in Nanomaterials (Basel, Switzerland), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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7 citing papers in PubMed.
- Tumor microenvironment responsive copper-doped carbon dots for synergistic chemotherapy and cuproptosis in laryngeal cancer.iScience · 2026Article
- Machine learning-enhanced identification of fluorophilic interactions for improved SERS detection of PFOA.Environmental science. Nano · 2026Article
- Metal-Organic Framework-Based Fluorinated Carbon for Li Primary Battery.Nanomaterials (Basel, Switzerland) · 2026Article
- Multifunctional PVDF membranes incorporating graphene, TiORSC advances · 2025Article
- Role of LiOH in Aqueous Electrocatalytic Defluorination of Perfluorooctanoic Sulfonate: Efficient Li-F Ion Pairing Prevents Anode Fouling by Produced Fluoride.ACS catalysis · 2024Article
- Electrochemical Performance of Niobium MXenes with Lanthanum.ACS applied materials & interfaces · 2024Article
- Transparent PDMS Surfaces with Covalently Attached Lubricants for Enhanced Anti-adhesion Performance.ACS applied materials & interfaces · 2024Article
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4 authors.
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Abstract
In this study, fluorinated graphene (FG) was synthesized via a hydrothermal reaction. Graphene oxides (GOs) with different oxygen bonding states and oxygen contents (GO(F), GO(P), and GO(HU)) were used as starting materials. GO(F) and GO(P) are commercial-type GOs from Grapheneall. GO(HU) was prepared using a modified Hummers method. The synthesized FGs from GO(F), GO(P), and GO(HU) are denoted as FG(F), FG(P), and FG(HU), respectively. The F atoms were bound to the graphene surface with predominantly semi-ionic or covalent bonding depending on the GO oxygen state. FG(F) and FG(HU) exhibited less extensive fluorination than FG(P) despite the same or higher oxygen contents compared with that in FG(P). This difference was attributed to the difference in the C=O content of GOs because the C=O bonds in GO primarily produce covalent C-F bonds. Thus, FG(F) and FG(HU) mainly exhibited semi-ionic C-F bonds. The doped F atoms were used to tune the electronic properties and surface chemistry of graphene. The fluorination reaction also improved the extent of reduction of GO.
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