ArticleNature materials2021
High-rate nanofluidic energy absorption in porous zeolitic frameworks.
Article in Nature materials, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 21 papers.
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Who cites it
21 citing papers in PubMed.
- Aerogel-involved triple-state viscoelastic fluidic materials enable high-efficiency dual-purpose energy management.Nature communications · 2026Article
- Crystallization-assisted water adsorption in amorphous molecular adsorbents.Nature communications · 2026Article
- Energetic and Structural Insights into Water Confined in Hydrophobic Nanopores.The journal of physical chemistry. C, Nanomaterials and interfaces · 2026Article
- Stable Compressible Liquids Made of Hierarchical MOF Nanocrystals.ACS applied materials & interfaces · 2025Article
- Integrated computational and experimental identification ofFrontiers in chemistry · 2025Article
- Water motifs in zirconium metal-organic frameworks induced by nanoconfinement and hydrophilic adsorption sites.Nature communications · 2024Article
- Screening Cu-Zeolites for Methane Activation Using Curriculum-Based Training.ACS catalysis · 2024Article
- Exploring the Heat of Water Intrusion into a Metal-Organic Framework by Experiment and Simulation.ACS applied materials & interfaces · 2024Article
- Fabrication of ZnO/ZnAlNanomaterials (Basel, Switzerland) · 2023Article
- Bimetallic Zeolitic Imidazole Frameworks for Improved Stability and Performance of Intrusion-Extrusion Energy Applications.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Challenges in modelling dynamic processes in realistic nanostructured materials at operating conditions.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2023Review
- Mechanism of Water Intrusion into Flexible ZIF-8: Liquid Is Not Vapor.Nano letters · 2023Article
- In situ micropillar compression of an anisotropic metal-organic framework single crystal.Communications chemistry · 2023Article
- Exploring the phase stability in interpenetrated diamondoid covalent organic frameworks.Communications chemistry · 2023Article
- High-Performance pH Sensor Electrodes Based on a Hexagonal Pt Nanoparticle Array-Coated Nanoporous Alumina Membrane.Materials (Basel, Switzerland) · 2022Article
- Effect of the Topology on Wetting and Drying of Hydrophobic Porous Materials.ACS applied materials & interfaces · 2022Article
- Vibrational Modes and Terahertz Phenomena of the Large-Cage Zeolitic Imidazolate Framework-71.The journal of physical chemistry letters · 2022Article
- Subnanometer Topological Tuning of the Liquid Intrusion/Extrusion Characteristics of Hydrophobic Micropores.Nano letters · 2022Article
- Review
- High-rate nanofluidic energy absorption in porous zeolitic frameworks.Nature materials · 2021Article
Corrections and comments
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Optimal mechanical impact absorbers are reusable and exhibit high specific energy absorption. The forced intrusion of liquid water in hydrophobic nanoporous materials, such as zeolitic imidazolate frameworks (ZIFs), presents an attractive pathway to engineer such systems. However, to harness their full potential, it is crucial to understand the underlying water intrusion and extrusion mechanisms under realistic, high-rate deformation conditions. Here, we report a critical increase of the energy absorption capacity of confined water-ZIF systems at elevated strain rates. Starting from ZIF-8 as proof-of-concept, we demonstrate that this attractive rate dependence is generally applicable to cage-type ZIFs but disappears for channel-containing zeolites. Molecular simulations reveal that this phenomenon originates from the intrinsic nanosecond timescale needed for critical-sized water clusters to nucleate inside the nanocages, expediting water transport through the framework. Harnessing this fundamental understanding, design rules are formulated to construct effective, tailorable and reusable impact energy absorbers for challenging new applications.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.