Evidence map›Paper›PMID 33863721›Full record

ArticleScience advances2021

Self-organization of nanoparticles and molecules in periodic Liesegang-type structures.

Amanda J Ackroyd, Gábor Holló, Haridas Mundoor, Honghu Zhang, Oleg Gang, Ivan I Smalyukh, István Lagzi, Eugenia Kumacheva

Open access · goldAbstract read
In one paragraph

Article in Science advances, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
2.9field-weighted citation impact, top 9% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed, 22 citations in OpenAlex.

  1. Article
  2. Article
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  4. Rapid formation of uniformly layered materials by coupling reaction-diffusion processes with mechanical responsiveness.Proceedings of the National Academy of Sciences of the United States of America · 2022
    Article
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors at 4 institutions in 4 countries.

Amanda J AckroydDepartment of Chemistry, University of Toronto, Toronto, ON M5S 3H6, Canada.ORCID http://orcid.org/0000-0001-6261-8701
Gábor HollóBME-MTA Condensed Matter Physics Research Group, Budapest H-1111, Hungary.ORCID http://orcid.org/0000-0001-9920-4801
Haridas MundoorDepartment of Physics, Materials Science and Engineering and Renewable and Sustainable Energy Institute (RASEI), University of Colorado, Boulder, CO 80309, USA.ORCID http://orcid.org/0000-0001-6589-6475
Honghu ZhangCenter for Functional Nanomaterials, Brookhaven National Laboratory, Upton, NY 11973, USA.
Oleg GangCenter for Functional Nanomaterials, Brookhaven National Laboratory, Upton, NY 11973, USA.ORCID http://orcid.org/0000-0001-5534-3121
Ivan I SmalyukhDepartment of Physics, Materials Science and Engineering and Renewable and Sustainable Energy Institute (RASEI), University of Colorado, Boulder, CO 80309, USA.ORCID http://orcid.org/0000-0003-3444-1966
István LagziCenter for Functional Nanomaterials, Brookhaven National Laboratory, Upton, NY 11973, USA. eugenia.kumacheva@utoronto.ca istvanlagzi@gmail.com.ORCID http://orcid.org/0000-0002-2303-5965
Eugenia KumachevaDepartment of Chemistry, University of Toronto, Toronto, ON M5S 3H6, Canada. eugenia.kumacheva@utoronto.ca istvanlagzi@gmail.com.ORCID http://orcid.org/0000-0001-5942-3890
Brookhaven National Laboratory · USUniversity of Colorado Boulder · USUniversity of Toronto · CAYukhnovskii Institute for Condensed Matter Physics of the National Academy of Sciences of Ukraine · UA

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Chemical organization in reaction-diffusion systems offers a strategy for the generation of materials with ordered morphologies and structural hierarchy. Periodic structures are formed by either molecules or nanoparticles. On the premise of new directing factors and materials, an emerging frontier is the design of systems in which the precipitation partners are nanoparticles and molecules. We show that solvent evaporation from a suspension of cellulose nanocrystals (CNCs) and l-(+)-tartaric acid [l-(+)-TA] causes phase separation and precipitation, which, being coupled with a reaction/diffusion, results in rhythmic alternation of CNC-rich and l-(+)-TA-rich rings. The CNC-rich regions have a cholesteric structure, while the l-(+)-TA-rich bands are formed by radially aligned elongated bundles. The moving edge of the pattern propagates with a finite constant velocity, which enables control of periodicity by varying film preparation conditions. This work expands knowledge about self-organizing reaction-diffusion systems and offers a strategy for the design of self-organizing materials.

Identifiers

PMID33863721
PMCPMC8051880
OpenAlexW3153526711

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC
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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.