ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2021
Analysis of the Ordering Effects in Anthraquinone Thin Films and Its Potential Application for Sodium Ion Batteries.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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10 citing papers in PubMed, 26 citations in OpenAlex.
- Evaluation of the Interphase-Related Cycling Stability of Thin-Film Amino- and Hydroxy-Substituted Anthraquinone Electrodes for Sodium-Ion Batteries.ACS applied energy materials · 2026Article
- Reversible Carbon Dioxide Capture and Release using an Electropolymerized Anthraquinone Electrode in Aqueous Solution.ACS applied materials & interfaces · 2025Article
- Effect of the Peri-Annulated Dichalcogenide Bridge on the Bipolar Character of Naphthalimide Derivatives Used as Organic Electrode Materials.Materials (Basel, Switzerland) · 2025Article
- Optimization of Zinc and Aluminum Hydroxyquinolines for Applications as Semiconductors in Molecular Electronics.Molecules (Basel, Switzerland) · 2025Article
- Characterization of the Coordination and Solvation Dynamics of Solvated Systems─Implications for the Analysis of Molecular Interactions in Solutions and Pure HJournal of chemical theory and computation · 2024Article
- Article
- How to use a rotating ring-disc electrode (RRDE) subtraction method to investigate the electrocatalytic oxygen reduction reaction?Catalysis science & technology · 2023Article
- Substantial Na-Ion Storage at High Current Rates: Redox-Pseudocapacitance through Sodium Oxide Formation.Nanomaterials (Basel, Switzerland) · 2022Article
- Direct Electrochemical COThe journal of physical chemistry. C, Nanomaterials and interfaces · 2022Article
- Anthraquinone and its derivatives as sustainable materials for electrochemical applications - a joint experimental and theoretical investigation of the redox potential in solution.Physical chemistry chemical physics : PCCP · 2022Article
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Authors and funding
9 authors at 5 institutions in 3 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The ordering effects in anthraquinone (AQ) stacking forced by thin-film application and its influence on dimer solubility and current collector adhesion are investigated. The structural characteristics of AQ and its chemical environment are found to have a substantial influence on its electrochemical performance. Computational investigation for different charged states of AQ on a carbon substrate obtained via basin hopping global minimization provides important insights into the physicochemical thin-film properties. The results reveal the ideal stacking configurations of the individual AQ-carrier systems and show ordering effects in a periodic supercell environment. The latter reveals the transition from intermolecular hydrogen bonding toward the formation of salt bridges between the reduced AQ units and a stabilizing effect upon the dimerlike rearrangement, while the strong surface-molecular interactions in the thin-film geometries are found to be crucial for the formed dimers to remain electronically active. Both characteristics, the improved current collector adhesion and the stabilization due to dimerization, are mutual benefits of thin-film electrodes over powder-based systems. This hypothesis has been further investigated for its potential application in sodium ion batteries. Our results show that AQ thin-film electrodes exhibit significantly better specific capacities (233 vs 87 mAh g
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