Evidence map›Paper›PMID 33624896›Full record

ArticleAdvanced materials (Deerfield Beach, Fla.)2021

In Situ Tracking of Wetting-Front Transient Heat Release on a Surface-Mounted Metal-Organic Framework.

Weijin Li, Guang Yang, Alexandros Terzis, Soumya Mukherjee, Chao He, Xingtao An, Jingyi Wu, Bernhard Weigand, Roland A Fischer

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In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors.

Weijin LiChair of Inorganic and Metal-Organic Chemistry, Catalysis Research Center, Ernst-Otto-Fischer Straße 1 and Department of Chemistry, Technical University of Munich, Lichtenbergstraße 4, Garching bei München, 85748, Germany.
Guang YangSchool of Mechanical Engineering, Shanghai Jiao Tong University, Dongchuan Road 800, Shanghai, 200240, China.
Alexandros TerzisDepartment of Mechanical Engineering, Stanford University, Stanford, CA, 94305, USA.
Soumya MukherjeeChair of Inorganic and Metal-Organic Chemistry, Catalysis Research Center, Ernst-Otto-Fischer Straße 1 and Department of Chemistry, Technical University of Munich, Lichtenbergstraße 4, Garching bei München, 85748, Germany.
Chao HeSchool of Sciences, Hebei University of Science and Technology, Yuxiang Street 26, Shijiazhuang, 050018, China.
Xingtao AnSchool of Sciences, Hebei University of Science and Technology, Yuxiang Street 26, Shijiazhuang, 050018, China.
Jingyi WuSchool of Mechanical Engineering, Shanghai Jiao Tong University, Dongchuan Road 800, Shanghai, 200240, China.
Bernhard WeigandInstitute of Aerospace Thermodynamics, University of Stuttgart, Pfaffenwaldring 31, Stuttgart, 70569, Germany.
Roland A FischerChair of Inorganic and Metal-Organic Chemistry, Catalysis Research Center, Ernst-Otto-Fischer Straße 1 and Department of Chemistry, Technical University of Munich, Lichtenbergstraße 4, Garching bei München, 85748, Germany.ORCID https://orcid.org/0000-0002-7532-5286

Funding

National Natural Science Foundation of China 51906142Shanghai Pujiang Program 19PJ1405600
6 · The paper itself

Abstract

Transient heat generation during guest adsorption and host-guest interactions is a natural phenomenon in metal-organic framework (MOF) chemistry. However, in situ tracking of such MOF released heat is an insufficiently researched field due to the fast heat dissipation to the surroundings. Herein, a facile capillary-driven liquid-imbibition approach is developed for in situ tracking of transient heat release at the wetting front of surface-mounted MOFs (SURMOFs) on cellulosic fiber substrates. Spatiotemporal temperature distributions are obtained with infrared thermal imaging for a range of MOF-based substrates and imbibed liquids. Temperature rises at the wetting front of water and binary mixtures with organic solvents are found to be over 10 K with an ultrafast and distinguishable thermal signal response (<1 s) with a detectable concentration limit ≤1 wt%. As an advancement to the state-of-the-art in trace-solvent detection technologies, this study shows great prospects for the integration of SURMOFs in future sensor devices. Inspired by this prototypal study, SURMOF-based transient heat signal transduction is likely to be extended to an ever-expanding library of SURMOFs and other classes of surface-grafted porous materials, translating into a wide range of convenient, portable, and ubiquitous sensor devices.

Indexed as

host-guest adsorptionliquid imbibitionmetal-organic framework thin filmssensor devicestransient heat

Identifiers

PMID33624896
PMCPMC11468584

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.