Evidence map›Paper›PMID 33606941›Full record

ArticleNano letters2021

Super-Resolution Mapping of a Chemical Reaction Driven by Plasmonic Near-Fields.

Ruben F Hamans, Matteo Parente, Andrea Baldi

Abstract read
In one paragraph

Article in Nano letters, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.

0numbers the graph read from it
0cells of the map it votes in
9citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

9 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Article
  5. Article
  6. Review
  7. Review
  8. Review
  9. Imaging and Localization of Single Emitters near Plasmonic Particles of Different Size, Shape, and Material.The journal of physical chemistry. C, Nanomaterials and interfaces · 2021
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

3 authors.

Ruben F HamansDutch Institute for Fundamental Energy Research, De Zaale 20, 5612 AJ Eindhoven, The Netherlands.
Matteo ParenteDutch Institute for Fundamental Energy Research, De Zaale 20, 5612 AJ Eindhoven, The Netherlands.
Andrea BaldiDutch Institute for Fundamental Energy Research, De Zaale 20, 5612 AJ Eindhoven, The Netherlands.ORCID http://orcid.org/0000-0001-9044-9378

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Plasmonic nanoparticles have recently emerged as promising photocatalysts for light-driven chemical conversions. Their illumination results in the generation of highly energetic charge carriers, elevated surface temperatures, and enhanced electromagnetic fields. Distinguishing between these often-overlapping processes is of paramount importance for the rational design of future plasmonic photocatalysts. However, the study of plasmon-driven chemical reactions is typically performed at the ensemble level and, therefore, is limited by the intrinsic heterogeneity of the catalysts. Here, we report an in situ single-particle study of a fluorogenic chemical reaction driven solely by plasmonic near-fields. Using super-resolution fluorescence microscopy, we map the position of individual product molecules with an ∼30 nm spatial resolution and demonstrate a clear correlation between the electric field distribution around individual nanoparticles and their super-resolved catalytic activity maps. Our results can be extended to systems with more complex electric field distributions, thereby guiding the design of future advanced photocatalysts.

Indexed as

fluorogenic reactionsnear-fieldsphotochemistryplasmonicssuper-resolution microscopy

Identifiers

PMID33606941
PMCPMC8023696

What OpenQuestion holds

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LicenceCC BY-NC-ND
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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.