ArticleNature communications2021
Thermodynamics of structure-forming systems.
Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Stochastic thermodynamics of social imitation beyond energetics.Nature communications · 2026Article
- Microscopic origin of abrupt mixed-order phase transitions.Nature communications · 2025Article
- Dissipative Self-Assembly of Patchy Particles under Nonequilibrium Drive: A Computational Study.Journal of chemical theory and computation · 2024Article
- The Typical Set and Entropy in Stochastic Systems with Arbitrary Phase Space Growth.Entropy (Basel, Switzerland) · 2023Article
- Equivalence of information production and generalised entropies in complex processes.PloS one · 2023Article
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Authors and funding
4 authors.
Funding
Abstract
Structure-forming systems are ubiquitous in nature, ranging from atoms building molecules to self-assembly of colloidal amphibolic particles. The understanding of the underlying thermodynamics of such systems remains an important problem. Here, we derive the entropy for structure-forming systems that differs from Boltzmann-Gibbs entropy by a term that explicitly captures clustered states. For large systems and low concentrations the approach is equivalent to the grand-canonical ensemble; for small systems we find significant deviations. We derive the detailed fluctuation theorem and Crooks' work fluctuation theorem for structure-forming systems. The connection to the theory of particle self-assembly is discussed. We apply the results to several physical systems. We present the phase diagram for patchy particles described by the Kern-Frenkel potential. We show that the Curie-Weiss model with molecule structures exhibits a first-order phase transition.
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Registered trials
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