Evidence map›Paper›PMID 33576576›Full record

ArticleChemSusChem2021

Sol-Gel Processing of Water-Soluble Carbon Nitride Enables High-Performance Photoanodes*.

Christiane Adler, Igor Krivtsov, Dariusz Mitoraj, Lucía Dos Santos-Gómez, Santiago García-Granda, Christof Neumann, Julian Kund, Christine Kranz, Boris Mizaikoff, Andrey Turchanin and 1 more

Open access · hybridAbstract read
In one paragraph

Article in ChemSusChem, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.

0numbers the graph read from it
0cells of the map it votes in
7citing papers in PubMed
1.1field-weighted citation impact, top 27% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

7 citing papers in PubMed, 29 citations in OpenAlex.

  1. Article
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  5. Operando IR Optical Control of Localized Charge Carriers in BiVOJournal of the American Chemical Society · 2023
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors at 3 institutions in 2 countries.

Christiane AdlerInstitute of Electrochemistry, Ulm University, Albert-Einstein-Allee 47, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0003-3063-738X
Igor KrivtsovInstitute of Electrochemistry, Ulm University, Albert-Einstein-Allee 47, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0003-4926-2338
Dariusz MitorajInstitute of Electrochemistry, Ulm University, Albert-Einstein-Allee 47, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0002-4285-5299
Lucía Dos Santos-GómezDepartment of Physical and Analytical Chemistry, University of Oviedo-CINN, 33006, Oviedo, Spain.ORCID http://orcid.org/0000-0002-1377-8351
Santiago García-GrandaDepartment of Physical and Analytical Chemistry, University of Oviedo-CINN, 33006, Oviedo, Spain.ORCID http://orcid.org/0000-0002-2373-0247
Christof NeumannInstitute of Physical Chemistry and Abbe Center of Photonics, Friedrich Schiller University Jena, Lessingstr. 10, 07743, Jena, Germany.ORCID http://orcid.org/0000-0002-3598-7656
Julian KundInstitute of Analytical and Bioanalytical Chemistry, Ulm University, Albert-Einstein-Allee 11, 89081, Ulm, Germany.
Christine KranzInstitute of Analytical and Bioanalytical Chemistry, Ulm University, Albert-Einstein-Allee 11, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0002-6001-0580
Boris MizaikoffInstitute of Analytical and Bioanalytical Chemistry, Ulm University, Albert-Einstein-Allee 11, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0002-5583-7962
Andrey TurchaninInstitute of Physical Chemistry and Abbe Center of Photonics, Friedrich Schiller University Jena, Lessingstr. 10, 07743, Jena, Germany.ORCID http://orcid.org/0000-0003-2388-1042
Radim BeranekInstitute of Electrochemistry, Ulm University, Albert-Einstein-Allee 47, 89081, Ulm, Germany.ORCID http://orcid.org/0000-0002-7926-0774
Universität Ulm · DEFriedrich Schiller University Jena · DEUniversidad de Oviedo · ES

Funding

Gobierno del Principado de Asturias GRUPIN-ID2018-170Spanish MINECO MAT2016-78155-C2-1-R
6 · The paper itself

Abstract

In spite of the enormous promise that polymeric carbon nitride (PCN) materials hold for various applications, the fabrication of high-quality, binder-free PCN films and electrodes has been a largely elusive goal to date. Here, we tackle this challenge by devising, for the first time, a water-based sol-gel approach that enables facile preparation of thin films based on poly(heptazine imide) (PHI), a polymer belonging to the PCN family. The sol-gel process capitalizes on the use of a water-soluble PHI precursor that allows formation of a non-covalent hydrogel. The hydrogel can be deposited on conductive substrates, resulting in formation of mechanically stable polymeric thin layers. The resulting photoanodes exhibit unprecedented photoelectrochemical (PEC) performance in alcohol reforming and highly selective (∼100 %) conversions with very high photocurrents (>0.25 mA cm

Indexed as

bias-free operationcarbon nitridephotoanodephotoelectrocatalysisphotoreforming

Identifiers

PMID33576576
PMCPMC8248241
OpenAlexW3112299391

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC-ND
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.