ArticleAdvanced materials (Deerfield Beach, Fla.)2021
Combination of Highly Efficient Electrocatalytic Water Oxidation with Selective Oxygenation of Organic Substrates using Manganese Borophosphates.
Article in Advanced materials (Deerfield Beach, Fla.), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed, 73 citations in OpenAlex.
- Dynamics in electrochemical organic oxidation reactions from in situ and operando techniques.Nature reviews. Chemistry · 2025Review
- Tailored Ni(OH)ACS applied materials & interfaces · 2024Article
- Immobilization of Oxyanions on the Reconstructed Heterostructure Evolved from a Bimetallic Oxysulfide for the Promotion of Oxygen Evolution Reaction.Nano-micro letters · 2023Article
- Challenges for Hybrid Water Electrolysis to Replace the Oxygen Evolution Reaction on an Industrial Scale.Global challenges (Hoboken, NJ) · 2023Article
- New Avenues to Chemical Space for Energy Materials by the Molecular Precursor Approach.Small science · 2023Article
- Perspective on intermetallics towards efficient electrocatalytic water-splitting.Chemical science · 2021Review
- Evolving Highly Active Oxidic Iron(III) Phase from Corrosion of Intermetallic Iron Silicide to Master Efficient Electrocatalytic Water Oxidation and Selective Oxygenation of 5-Hydroxymethylfurfural.Advanced materials (Deerfield Beach, Fla.) · 2021Article
- Combination of Highly Efficient Electrocatalytic Water Oxidation with Selective Oxygenation of Organic Substrates using Manganese Borophosphates.Advanced materials (Deerfield Beach, Fla.) · 2021Article
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Authors and funding
9 authors at 3 institutions in 2 countries.
Funding
Abstract
One of the key catalytic reactions for life on earth, the oxidation of water to molecular oxygen, occurs in the oxygen-evolving complex of the photosystem II (PSII) mediated by a manganese-containing cluster. Considerable efforts in this research area embrace the development of efficient artificial manganese-based catalysts for the oxygen evolution reaction (OER). Using artificial OER catalysts for selective oxygenation of organic substrates to produce value-added chemicals is a worthwhile objective. However, unsatisfying catalytic performance and poor stability have been a fundamental bottleneck in the field of artificial PSII analogs. Herein, for the first time, a manganese-based anode material is developed and paired up for combining electrocatalytic water oxidation and selective oxygenations of organics delivering the highest efficiency reported to date. This can be achieved by employing helical manganese borophosphates, representing a new class of materials. The uniquely high catalytic activity and durability (over 5 months) of the latter precursors in alkaline media are attributed to its unexpected surface transformation into an amorphous MnO
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