Evidence map›Paper›PMID 33469009›Full record

ArticleNature communications2021

Floquet spin states in OLEDs.

S Jamali, V V Mkhitaryan, H Malissa, A Nahlawi, H Popli, T Grünbaum, S Bange, S Milster, D M Stoltzfus, A E Leung and 4 more

Abstract read
In one paragraph

Article in Nature communications, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Floquet States of Chemoselective Alternating Current Electrosynthesis.Journal of the American Chemical Society · 2026
    Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

S Jamali *Department of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA.
V V Mkhitaryan *Department of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA.
H MalissaDepartment of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA.ORCID http://orcid.org/0000-0002-5964-3225
A NahlawiDepartment of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA.
H PopliDepartment of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA.
T GrünbaumInstitut für Experimentelle und Angewandte Physik, Universität Regensburg, 93053, Regensburg, Germany.
S BangeInstitut für Experimentelle und Angewandte Physik, Universität Regensburg, 93053, Regensburg, Germany.ORCID http://orcid.org/0000-0002-5850-264X
S MilsterInstitut für Experimentelle und Angewandte Physik, Universität Regensburg, 93053, Regensburg, Germany.
D M StoltzfusCentre for Organic Photonics & Electronics, School of Chemistry and Molecular Biosciences, The University of Queensland, Brisbane, QLD, 4072, Australia.
A E LeungNational Deuteration Facility, Australian Nuclear Science and Technology Organization (ANSTO), Lucas Heights, NSW, 2234, Australia.
T A DarwishNational Deuteration Facility, Australian Nuclear Science and Technology Organization (ANSTO), Lucas Heights, NSW, 2234, Australia.
P L BurnCentre for Organic Photonics & Electronics, School of Chemistry and Molecular Biosciences, The University of Queensland, Brisbane, QLD, 4072, Australia.ORCID http://orcid.org/0000-0003-3405-3517
J M LuptonDepartment of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA. john.lupton@ur.de.ORCID http://orcid.org/0000-0002-7899-7598
C BoehmeDepartment of Physics and Astronomy, University of Utah, Salt Lake City, UT, 84112, USA. boehme@physics.utah.edu.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Electron and hole spins in organic light-emitting diodes constitute prototypical two-level systems for the exploration of the ultrastrong-drive regime of light-matter interactions. Floquet solutions to the time-dependent Hamiltonian of pairs of electron and hole spins reveal that, under non-perturbative resonant drive, when spin-Rabi frequencies become comparable to the Larmor frequencies, hybrid light-matter states emerge that enable dipole-forbidden multi-quantum transitions at integer and fractional g-factors. To probe these phenomena experimentally, we develop an electrically detected magnetic-resonance experiment supporting oscillating driving fields comparable in amplitude to the static field defining the Zeeman splitting; and an organic semiconductor characterized by minimal local hyperfine fields allowing the non-perturbative light-matter interactions to be resolved. The experimental confirmation of the predicted Floquet states under strong-drive conditions demonstrates the presence of hybrid light-matter spin excitations at room temperature. These dressed states are insensitive to power broadening, display Bloch-Siegert-like shifts, and are suggestive of long spin coherence times, implying potential applicability for quantum sensing.

Identifiers

PMID33469009
PMCPMC7815916

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.