ArticleAngewandte Chemie (International ed. in English)2021
Ruthenium-Catalyzed Dehydrogenation Through an Intermolecular Hydrogen Atom Transfer Mechanism.
Article in Angewandte Chemie (International ed. in English), 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Mechanistic Insights on Fe(II)-Catalyzed Depolymerization of Poly(Ethylene Terephthalate) by Transesterification.Chemistry, an Asian journal · 2026Article
- Site-Selective Benzylic Dehydrogenation of Alkylindoles.JACS Au · 2025Article
- Tandem dehydrogenation-olefination-decarboxylation of cycloalkyl carboxylic acids via multifold C-H activation.Nature communications · 2024Article
- Multiple remote C(spChemical science · 2022Article
- Homogenous Cr and C Doped 3D Self-Supporting NiO Cellular Nanospheres for Hydrogen Evolution Reaction.Materials (Basel, Switzerland) · 2022Article
- Selective desaturation of amides: a direct approach to enamides.Chemical science · 2022Article
- Cobalt-catalyzed chemoselective dehydrogenation through radical translocation under visible light.Chemical science · 2022Article
- Direct Synthesis of Enamides via Electrophilic Activation of Amides.Journal of the American Chemical Society · 2021Article
- Ruthenium-Catalyzed Dehydrogenation Through an Intermolecular Hydrogen Atom Transfer Mechanism.Angewandte Chemie (International ed. in English) · 2021Article
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Authors and funding
5 authors.
Funding
Abstract
The direct dehydrogenation of alkanes is among the most efficient ways to access valuable alkene products. Although several catalysts have been designed to promote this transformation, they have unfortunately found limited applications in fine chemical synthesis. Here, we report a conceptually novel strategy for the catalytic, intermolecular dehydrogenation of alkanes using a ruthenium catalyst. The combination of a redox-active ligand and a sterically hindered aryl radical intermediate has unleashed this novel strategy. Importantly, mechanistic investigations have been performed to provide a conceptual framework for the further development of this new catalytic dehydrogenation system.
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Registered trials
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