ArticleProceedings of the National Academy of Sciences of the United States of America2021
Gigantic vortical differential scattering as a monochromatic probe for multiscale chiral structures.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 27 papers.
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Who cites it
27 citing papers in PubMed.
- Nonlinear directional emission on monolayer MoSScience advances · 2026Article
- Dual-parameter chiral detection at the single-particle level enabled by surface cosine waves.Science advances · 2026Article
- Vortical Differential Scattering of Spatio-Temporal Optical Vortex With Arbitrarily Oriented Orbital Angular Momentum by Chiral Spherical Particle.Nanophotonics (Berlin, Germany) · 2026Article
- Multidimensional helical dichroism from a chiral molecular nanoassembly.Nature communications · 2026Article
- Observation of strong spin-orbit couplings in plasmonic spin-twistronics topological lattices.Nature communications · 2026Article
- Quantum-elevated chiral discrimination for biomolecules.Science advances · 2026Article
- Gigantic Vortical Dichroism and Handedness-Dependent Optical Response in Spiral Metamaterials.Nanomaterials (Basel, Switzerland) · 2026Article
- Spin angular momentum modulation via spin-orbit interaction in fractional orbital angular momentum beams.Nanophotonics (Berlin, Germany) · 2025Article
- Research on the Generation of High-Purity Vortex Beams Aided by Genetic Algorithms.Nanomaterials (Basel, Switzerland) · 2025Article
- Optical Activity Modulation in Chiral Metasurfaces via Structured Light.Nano letters · 2025Article
- Strong Chiro-Optical Activity of Plasmonic Metasurfaces with Inverted Pyramid Arrays.ACS applied materials & interfaces · 2025Article
- Giant Helical Dichroism in Twisted Hollow-Core Photonic Crystal Fibers.ACS photonics · 2025Article
- Compact and reciprocal probe-signal-integrated rotational Doppler velocimetry with fiber-sculpted light.Light, science & applications · 2025Article
- Simultaneous control of three degrees of freedom in perfect vector vortex beams based on metasurfaces.Nanophotonics (Berlin, Germany) · 2025Article
- Giant Vortex Dichroism in Simplified-Chiral-Double-Elliptical Metamaterials.Nanomaterials (Basel, Switzerland) · 2025Article
- Simultaneous generation of first- to fourth-order OAM modes based on a cascaded preset-twist long-period fiber grating.Nanophotonics (Berlin, Germany) · 2024Article
- Harnessing spin and orbital angular momentum light for optimal algae growth.Scientific reports · 2024Article
- Dense Space-Division Multiplexing Exploiting Multi-Ring Perfect Vortex.Sensors (Basel, Switzerland) · 2023Article
- Metafiber transforming arbitrarily structured light.Nature communications · 2023Article
- Geometric Phase in Twisted Topological Complementary Pair.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
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Authors and funding
13 authors.
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No grant is acknowledged in the PubMed record.
Abstract
Spin angular momentum of light is vital to investigate enantiomers characterized by circular dichroism (CD), widely adopted in biology, chemistry, and material science. However, to discriminate chiral materials with multiscale features, CD spectroscopy normally requires wavelength-swept laser sources as well as wavelength-specific optical accessories. Here, we experimentally demonstrate an orbital-angular-momentum-assisted approach to yield chiroptical signals with monochromatic light. The gigantic vortical differential scattering (VDS) of ∼120% is achieved on intrinsically chiral microstructures fabricated by femtosecond laser. The VDS measurements can robustly generate chiroptical properties on microstructures with varying geometric features (e.g., diameters and helical pitches) and detect chiral molecules with high sensitivity. This VDS scheme lays a paradigm-shift pavement toward efficiently chiroptical discrimination of multiscale chiral structures with photonic orbital angular momentum. It simplifies and complements the conventional CD spectroscopy, opening possibilities for measuring weak optical chirality, especially on mesoscale chiral architectures and macromolecules.
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