ArticleThe journal of physical chemistry. B2021
Confined Water Molecules in Binary Mixtures of Water and 2,6-Lutidine Near Lower Solution Critical Temperature.
Article in The journal of physical chemistry. B, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed, 5 citations in OpenAlex.
- Direct Probing of Vibrational Interactions in UiO-66 Polycrystalline Membranes with Femtosecond Two-Dimensional Infrared Spectroscopy.The journal of physical chemistry letters · 2022Article
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Authors and funding
2 authors at 1 institution in 1 country.
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Abstract
We study the concentration and temperature dependence of the reorientation dynamics of water molecules in binary mixtures of water and 2,6-lutidine below the lower solution critical temperature (LSCT) with femtosecond mid-infrared pump-probe spectroscopy. The measurements reveal the presence of water molecules interacting with both the hydrophobic groups of lutidine and forming a hydrogen bond with the nitrogen atom of lutidine. Both types of molecules show a strongly decreased rotational mobility in comparison to bulk water. From the temperature dependence of the slow water fraction, we conclude that the lutidine molecules form clusters that decrease in size when the temperature is decreased further below the LSCT.
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