ArticleFrontiers in chemistry2020
Tunable Non-linear Refraction Properties and Ultrafast Excited State Dynamics of Dicyanomethylene Dihydrofuran Derivative.
Article in Frontiers in chemistry, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed.
- Complex and Unusual Excited-State Relaxation Dynamics of 9,9'-Bifluorenylidene Revealed by Comprehensive Time-Resolved Spectroscopy and MRSF-TDDFT Calculations.The journal of physical chemistry letters · 2026Article
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7 authors.
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Abstract
The third order non-linear optical response of a dicyanomethylene dihydrofuran compound (DCDHF-2V) was investigated using a Z-scan technique in picosecond and nanosecond time regimes. The results show that DCDHF-2V has excellent excited state non-linear refraction properties on both time regimes, and the non-linear refraction index is also solvent-dependent in the nanosecond regime. The excited state relaxation dynamics of DCDHF-2V were demystified via femtosecond transient absorption spectroscopy. The TA spectra reveal that the solvent viscosities have a substantial impact on the excited state relaxation of DCDHF-2V. The exotic photophysical phenomena in DCDHF-2V reported herein can shed new light on future development of small organic non-linear optical materials with large non-linear coefficients and fast response.
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