ArticleNature communications2020
Vibrational couplings and energy transfer pathways of water's bending mode.
Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 35 papers.
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Who cites it
35 citing papers in PubMed.
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- Collapse of the Helical Hydrogen Bond Structure in Imidazolium HydrogenThe journal of physical chemistry letters · 2026Article
- Synergistic Enhancement of Polymer-Cement Waterproof Coatings by Silane-Functionalized Cellulose Nanofibril.Materials (Basel, Switzerland) · 2026Article
- Amphidynamic Molecular Crystal with Temperature-Controlled Helical Hydrogen-Bonded Network: Proton Dynamics and Order-Disorder Phase Transition.The journal of physical chemistry letters · 2026Article
- Altered morphology and diffusivity of water confined in MXenes: Machine learning-accelerated computations combined with experiments.Science advances · 2026Article
- Measurement of a Preresonant Hyper-Raman Hyperpolarizability.The journal of physical chemistry letters · 2026Article
- Real-time tracking of the intramolecular vibrational dynamics of liquid water.Communications chemistry · 2026Article
- Steric and hydrophilic/hydrophobic effects of organic cations on electrochemical CO reduction.Nature communications · 2025Article
- Electrical Conductivity and Permittivity of Porous Media: Origin, Measurements, and Implications.ACS measurement science au · 2025Review
- Efficient oxidative degradation of Azo dyes by cobalt(II) porphyrin complex supported on modified bentonite and chitosan: structural characterization and mechanistic insight.Scientific reports · 2025Article
- Magnetic Field-Driven Interface Hydroxylation via the Vibrational Stark Effect Boosts Alkaline Hydrogen Evolution Reaction.JACS Au · 2025Article
- Tailored Magnetic FeDiagnostics (Basel, Switzerland) · 2025Article
- Theoretical and quantum mechanical deconstruction of vibrational energy transfer pathways modified by collective vibrational strong coupling.Nature communications · 2025Article
- The Transcription Machinery and the Driving Force of the Transcriptional Molecular Condensate: The Role of Phosphates.Current issues in molecular biology · 2025Article
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- Decoding Double Layer Dynamics forAngewandte Chemie (International ed. in English) · 2025Article
- Microheterogeneity in Liquid Water Associated with Hydrogen-Bond Cooperativity-IR Spectroscopic and MD Simulation Study of Temperature Effect.International journal of molecular sciences · 2025Article
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Authors and funding
11 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Coupling between vibrational modes is essential for energy transfer and dissipation in condensed matter. For water, different O-H stretch modes are known to be very strongly coupled both within and between water molecules, leading to ultrafast dissipation and delocalization of vibrational energy. In contrast, the information on the vibrational coupling of the H-O-H bending mode of water is lacking, even though the bending mode is an essential intermediate for the energy relaxation pathway from the stretch mode to the heat bath. By combining static and femtosecond infrared, Raman, and hyper-Raman spectroscopies for isotopically diluted water with ab initio molecular dynamics simulations, we find the vibrational coupling of the bending mode differs significantly from the stretch mode: the intramode intermolecular coupling of the bending mode is very weak, in stark contrast to the stretch mode. Our results elucidate the vibrational energy transfer pathways of water. Specifically, the librational motion is essential for the vibrational energy relaxation and orientational dynamics of H-O-H bending mode.
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